Superstructures with Atomic-Level Arranged Perovskite and Oxide Layers for Advanced Oxidation with an Enhanced Non-Free Radical Pathway

Article

Yang, Li, Jiao, Yong, Xu, Xiaomin, Pan, Yangli, Su, Chao, Duan, Xiaoguang, Sun, Hongqi, Liu, Shaomin, Wang, Shaobin and Shao, Zongping. 2022. "Superstructures with Atomic-Level Arranged Perovskite and Oxide Layers for Advanced Oxidation with an Enhanced Non-Free Radical Pathway." ACS Sustainable Chemistry and Engineering. 10 (5), pp. 1899-1909. https://doi.org/10.1021/acssuschemeng.1c07605
Article Title

Superstructures with Atomic-Level Arranged Perovskite and Oxide Layers for Advanced Oxidation with an Enhanced Non-Free Radical Pathway

ERA Journal ID200101
Article CategoryArticle
AuthorsYang, Li, Jiao, Yong, Xu, Xiaomin, Pan, Yangli, Su, Chao, Duan, Xiaoguang, Sun, Hongqi, Liu, Shaomin, Wang, Shaobin and Shao, Zongping
Journal TitleACS Sustainable Chemistry and Engineering
Journal Citation10 (5), pp. 1899-1909
Number of Pages11
Year2022
PublisherAmerican Chemical Society
Place of PublicationUnited States
ISSN2168-0485
Digital Object Identifier (DOI)https://doi.org/10.1021/acssuschemeng.1c07605
Web Address (URL)https://pubs.acs.org/doi/10.1021/acssuschemeng.1c07605
Abstract

Perovskite-based oxides demonstrate a great catalytic efficiency in advanced oxidation processes (AOPs), where both free and non-free radical pathways may occur. The non-free radical pathway is preferable because it is less affected by the wastewater environment, yet little is known about its origin. Here, we exploit Ruddlesden–Popper (RP) layered perovskite oxides as an excellent platform for investigating the structure–property relationship for peroxymonosulfate (PMS) activation in AOPs. The atomic-level interaction of the perovskite and rock salt layers in RP oxides stabilizes the transition metals at low valences, causing the formation of abundant lattice oxygen/interstitial oxygen species. Unlike oxygen vacancies in conventional perovskites, which promote free-radical generation, these reactive oxygen species in RP perovskites have high activity and mobility and facilitate the formation of non-free radical singlet oxygen. This singlet oxygen reaction pathway is optimized by tailoring the oxygen species, leading to the discovery of LaSrCo0.8Fe0.2O4 with exceptionally efficient PMS activation.

Keywordsinterstitial oxygen; Ruddlesden−Popper layered perovskite; non-free radical pathway; reactive oxygen species; peroxymonosulfate
ANZSRC Field of Research 20204004. Chemical engineering
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Byline AffiliationsNanjing Tech University, China
Curtin University
Centre for Future Materials
Jiangsu University of Science and Technology, China
University of Adelaide
Edith Cowan University
Curtin University of Technology
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Synthesis and characterization of three amino-functionalized metal–organic frameworks based on the 2-aminoterephthalic ligand
Yang, Ying, Lin, Rijia, Ge, Lei, Hou, Lei, Bernhardt, Paul, Rufford, Thomas E., Wang, Shaobin, Rudolph, Victor, Wang, Yaoyu and Zhu, Zhonghua. 2015. "Synthesis and characterization of three amino-functionalized metal–organic frameworks based on the 2-aminoterephthalic ligand." Dalton Transactions: an international journal of inorganic chemistry. 44 (17), pp. 8190-8197. https://doi.org/10.1039/C4DT03927K
Amphiphobic PVDF composite membranes for anti-fouling direct contact membrane distillation
Lu, Xuemei, Peng, Yuelian, Ge, Lei, Lin, Rijia, Zhu, Zhonghua and Liu, Shaomin. 2016. "Amphiphobic PVDF composite membranes for anti-fouling direct contact membrane distillation." Journal of Membrane Science. 505, pp. 61-69. https://doi.org/10.1016/j.memsci.2015.12.042