Catalytic partial oxidation of methane to syngas: review of perovskite catalysts and membrane reactors
Article
Elbadawi, Abdalwadood H, Ge, Lei, Li, Zhiheng, Liu, Shaomin, Wang, Shaobin and Zhu, Zhonghua. 2021. "Catalytic partial oxidation of methane to syngas: review of perovskite catalysts and membrane reactors." Catalysis Reviews: Science and Engineering. 63 (1), pp. 1-67. https://doi.org/10.1080/01614940.2020.1743420
Article Title | Catalytic partial oxidation of methane to syngas: review of perovskite catalysts and membrane reactors |
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ERA Journal ID | 1415 |
Article Category | Article |
Authors | Elbadawi, Abdalwadood H, Ge, Lei, Li, Zhiheng, Liu, Shaomin, Wang, Shaobin and Zhu, Zhonghua |
Journal Title | Catalysis Reviews: Science and Engineering |
Journal Citation | 63 (1), pp. 1-67 |
Number of Pages | 67 |
Year | 2021 |
Publisher | Taylor & Francis |
Place of Publication | United States |
ISSN | 0161-4940 |
1520-5703 | |
Digital Object Identifier (DOI) | https://doi.org/10.1080/01614940.2020.1743420 |
Web Address (URL) | https://www.tandfonline.com/doi/full/10.1080/01614940.2020.1743420 |
Abstract | Partial oxidation of methane (POM) offers a promising option to produce syngas for downstream processes such as hydrogen production and Fischer-Tropsch processes. POM in fixed-bed reactors requires an oxygen separation plant with high operation cost and safety risks. On the contrary, membrane reactors can provide an improved process by integrating both oxygen separation and catalytic reaction processes. With many advantages including high purity and efficient oxygen separation from the air at the catalytic reaction conditions, mixed ionic-electronic conducting membranes (MIEC) caught great attention in the scientific research field over the past two decades. In this review, POM using different catalysts in fixed-bed reactors was firstly summarized with emphasizing on perovskite-based catalysts, and then the material screening of MIEC membrane reactors was introduced and linked to the selection of conventional and perovskite catalysts. The catalytic activity, reaction mechanisms, and emerging challenges have been analyzed. Furthermore, future research directions have been outlined by highlighting the effect of electronic properties, continuous reduction-oxidation in the presence of oxygen flux, and chemical reaction mechanism on membrane/catalyst. © 2020 Taylor & Francis. |
Keywords | mechanism; Partial oxidation; syngas; membrane reactors |
Contains Sensitive Content | Does not contain sensitive content |
ANZSRC Field of Research 2020 | 340601. Catalysis and mechanisms of reactions |
Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
Byline Affiliations | University of Queensland |
Centre for Future Materials | |
Beijing University of Chemical Technology, China | |
University of Adelaide |
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