New Insights into the Degradation Behavior of Air Electrodes during Solid Oxide Electrolysis and Reversible Solid Oxide Cell Operation
Article
Khan, Muhammad Shirjeel, Xu, Xiaoyong, Knibbe, Ruth, Rehman, Ateeq Ur, Li, Zhiheng, Yago, Anya Josefa, Wang, Hao and Zhu, Zhonghua. 2020. "New Insights into the Degradation Behavior of Air Electrodes during Solid Oxide Electrolysis and Reversible Solid Oxide Cell Operation
." Energy Technology: generation, conversion, storage, distribution. 8 (9). https://doi.org/10.1002/ente.202000241
| Article Title | New Insights into the Degradation Behavior of Air Electrodes during Solid Oxide Electrolysis and Reversible Solid Oxide Cell Operation |
|---|---|
| ERA Journal ID | 200427 |
| Article Category | Article |
| Authors | Khan, Muhammad Shirjeel, Xu, Xiaoyong, Knibbe, Ruth, Rehman, Ateeq Ur, Li, Zhiheng, Yago, Anya Josefa, Wang, Hao and Zhu, Zhonghua |
| Journal Title | Energy Technology: generation, conversion, storage, distribution |
| Journal Citation | 8 (9) |
| Article Number | 2000241 |
| Number of Pages | 10 |
| Year | 2020 |
| Publisher | John Wiley & Sons |
| Place of Publication | Germany |
| ISSN | 2194-4288 |
| 2194-4296 | |
| Digital Object Identifier (DOI) | https://doi.org/10.1002/ente.202000241 |
| Web Address (URL) | https://onlinelibrary-wiley-com.ezproxy.usq.edu.au/doi/full/10.1002/ente.202000241 |
| Abstract | The commercialization of reversible solid oxide cells (RSOCs) is limited by the severe degradation of the air electrodes during solid oxide electrolysis cells (SOECs) operation. Herein, the degradation behavior of (La0.8Sr0.2)0.95Mn1−xCoxO3−δ (LSMC) air electrodes where x = 0.1, 0.3, and 0.5 is reported. After the SOEC test, the air electrode with x = 0.1 delaminates. While previous studies reported delamination due to the disintegration of air electrodes, for the first time, it is shown that delamination can also occur due to the disintegration of the samaria-doped ceria (SDC) barrier layer into nanoparticles. The formation of such nanoparticles weakens the contact between the air electrode and barrier layer and encourages delamination. The air electrode with x = 0.3, shows excellent long-term stability and also produces an electrolysis current density of 0.63 A cm−2 in 50% H2O/50% H2 at 1.3 V. This mechanistic study will allow researchers to develop air electrodes with improved long-term stability. |
| Keywords | delamination; interfaces; oxygen partial pressures; reversible solid oxide cells |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401602. Composite and hybrid materials |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | University of Queensland |
| Centre for Future Materials |
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Li, Mengran, Idros, Mohamed Nazmi, Wu, Yuming, Garg, Sahil, Gao, Shuai, Lin, Rijia, Rabiee, Hesamoddin, Li, Zhiheng, Ge, Lei, Rufford, Thomas Edward, Zhu, Zhonghua, Li, Liye and Wang, Geoff. 2021. "Unveiling the effects of dimensionality of tin oxide-derived catalysts on CO2 reduction by using gas-diffusion electrodes." Reaction Chemistry and Engineering. 6 (2), pp. 345-352. https://doi.org/10.1039/D0RE00396DOne-Pot, Solvent- and Catalyst-Free Synthesis of Polyphosphoramide as an Eco-Benign and Effective Flame Retardant for Poly(lactic acid)
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Wang, Jing-Gang, Zhang, Xiao-Qing, Sheng, Ang, Zhu, Jin, Song, Ping-An, Wang, Hao and Liu, Xiao-Qing. 2020. "Synthesis and Properties Investigation of Thiophene-aromatic Polyesters: Potential Alternatives for the 2,5-Furandicarboxylic Acid-based Ones." Chinese Journal of Polymer Science. 38, pp. 1082-1091. https://doi.org/10.1007/s10118-020-2438-2Revealing cracking and breakage behaviours of gibbsite particles
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Yang, Haitang, Yu, Bin, Xu, Xiaodong, Bourbigot, Serge, Wang, Hao and Song, Pingan. 2020. "Lignin-derived bio-based flame retardants toward high-performance sustainable polymeric materials." Green Chemistry. 22 (7), pp. 2129-2161. https://doi.org/10.1039/D0GC00449AManipulating interphase reactions for mechanically robust, flame-retardant and sustainable polylactide biocomposites
Xu, Xiaodong, Dai, Jinfeng, Ma, Zhewen, Liu, Lina, Zhang, Xinghong, Liu, Hongzhi, Tang, Long-Cheng, Huang, Guobo, Wang, Hao and Song, Pingan. 2020. "Manipulating interphase reactions for mechanically robust, flame-retardant and sustainable polylactide biocomposites." Composites Part B: Engineering. 190, pp. 1-15. https://doi.org/10.1016/j.compositesb.2020.107930Grafting Lignin with Bioderived Polyacrylates for Low-Cost, Ductile, and Fully Biobased Poly(lactic acid) Composite
Sun, Yiqi, Ma, Zhewen, Xu, Xiaodong, Liu, Xiaohuan, Liu, Lina, Huang, Guobo, Liu, Lei, Wang, Hao and Song, Pingan. 2020. "Grafting Lignin with Bioderived Polyacrylates for Low-Cost, Ductile, and Fully Biobased Poly(lactic acid) Composite." ACS Sustainable Chemistry and Engineering. 8 (5), pp. 2267-2276. https://doi.org/10.1021/acssuschemeng.9b06593Realizing simultaneous improvements in mechanical strength, flame retardancy and smoke suppression of ABS nanocomposites from multifunctional graphene
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Yang, Haitang, Yu, Bin, Song, Pingan, Maluk, Cristian and Wang, Hao. 2019. "Surface-coating engineering for flame retardant flexible polyurethane foams: A critical review." Composites Part B: Engineering. 176, pp. 1-14. https://doi.org/10.1016/j.compositesb.2019.107185Synthesis of decorated graphene with P, N-containing compounds and its flame retardancy and smoke suppression effects on polylactic acid
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Fang, Fang, Ran, Shiya, Fang, Zhengping, Song, Pingan and Wang, Hao. 2019. "Improved flame resistance and thermo-mechanical properties of epoxy resin nanocomposites from functionalized graphene oxide via self-assembly in water." Composites Part B: Engineering. 165, pp. 406-416. https://doi.org/10.1016/j.compositesb.2019.01.086One-pot scalable fabrication of an oligomeric phosphoramide towards high-performance flame retardant polylactic acid with a submicron-grained structure
Xue, Yijiao, Shen, Mingxia, Zheng, Yifei, Tao, Wenzhu, Han, Yanxin, Li, Weidong, Song, Pingan and Wang, Hao. 2020. "One-pot scalable fabrication of an oligomeric phosphoramide towards high-performance flame retardant polylactic acid with a submicron-grained structure." Composites Part B: Engineering. 183, pp. 1-12. https://doi.org/10.1016/j.compositesb.2019.107695A bio-based ionic complex with different oxidation states of phosphorus for reducing flammability and smoke release of epoxy resins
Fang, Fang, Huo, Siqi, Shen, Haifeng, Ran, Shiya, Wang, Hao, Song, Pingan and Fang, Zhengping. 2020. "A bio-based ionic complex with different oxidation states of phosphorus for reducing flammability and smoke release of epoxy resins." Composites Communications. 17, pp. 104-108. https://doi.org/10.1016/j.coco.2019.11.011High‐performance polymeric materials through hydrogen‐bond cross‐linking
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Wang, Lijun, Hong, Min, Kawami, Youichirou, Sun, Qiang, Nguyen, Van Thuong, Wang, Yuan, Yue, Luo, Zheng, Shuqi, Zhu, Zhonghua, Zou, Jin and Chen, Zhi-Gang. 2020. "Crowding-out effect strategy using AgCl for realizing a super low lattice thermal conductivity of SnTe." Sustainable Materials and Technologies. 25, pp. 1-7. https://doi.org/10.1016/j.susmat.2020.e00183Tuning the Product Selectivity of the Cu Hollow Fiber Gas Diffusion Electrode for Efficient CO2 Reduction to Formate by Controlled Surface Sn Electrodeposition
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Elbadawi, Abdalwadood H, Ge, Lei, Li, Zhiheng, Liu, Shaomin, Wang, Shaobin and Zhu, Zhonghua. 2021. "Catalytic partial oxidation of methane to syngas: review of perovskite catalysts and membrane reactors." Catalysis Reviews: Science and Engineering. 63 (1), pp. 1-67. https://doi.org/10.1080/01614940.2020.1743420A thermally insulating vermiculite nanosheet-epoxy nanocomposite paint as a fire-resistant wood coating
Sethurajaperumal, Abimannan, Manohar, Anagha, Banerjee, Arghya, Varrla, Eswaraiah, Wang, Hao and Ostrikov, Kostya (Ken). 2021. "A thermally insulating vermiculite nanosheet-epoxy nanocomposite paint as a fire-resistant wood coating." Nanoscale Advances. 3 (14), pp. 4235-4243. https://doi.org/10.1039/d1na00207dEnhanced toughness of PLLA/PCL blends using poly(d-lactide)-poly(ε-caprolactone)-poly(d-lactide) as compatibilizer
Xiao, Xianglian, Chevali, Venkata S., Song, Pingan, Yu, Bin, Yang, Yihu and Wang, Hao. 2020. "Enhanced toughness of PLLA/PCL blends using poly(d-lactide)-poly(ε-caprolactone)-poly(d-lactide) as compatibilizer." Composites Communications. 21, pp. 1-6. https://doi.org/10.1016/j.coco.2020.100385Direct evidence of boosted oxygen evolution over perovskite by enhanced lattice oxygen participation
Pan, Yangli, Xu, Xiaomin, Zhong, Yijun, Ge, Lei, Chen, Yubo, Veder, Jean-Pierre Marcel, Guan, Daqin, O’Hayre, Ryan, Li, Mengran, Wang, Guoxiong, Wang, Hao, Zhou, Wei and Shao, Zongping. 2020. "Direct evidence of boosted oxygen evolution over perovskite by enhanced lattice oxygen participation." Nature Communications. 11, pp. 1-10. https://doi.org/10.1038/s41467-020-15873-xCurrent status of carbon fibre and carbon fibre composites recycling
Zhang, Jin, Chevali, Venkata S., Wang, Hao and Wang, Chun-Hui. 2020. "Current status of carbon fibre and carbon fibre composites recycling." Composites Part B: Engineering. 193, pp. 1-15. https://doi.org/10.1016/j.compositesb.2020.108053Interfacial engineering of polymer-MOF composite by in situ vitrification
Lin, Rijia, Hou, Jingwei, Li, Mengran, Wang, Zhanke, Ge, Lei, Li, Shichun, Smart, Simon, Zhu, Zhonghua, Bennett, Thomas D. and Chen, Vicki. 2020. "Interfacial engineering of polymer-MOF composite by in situ vitrification." Chemical Communications. 56 (25), pp. 3609-3612. https://doi.org/10.1039/d0cc00664eCracking behaviour and mechanism at grain boundary of gibbsite during calcination
Zhang, Jinxuan, Ge, Lei, Chen, Zhi-Gang and Zhu, Zhonghua. 2020. "Cracking behaviour and mechanism at grain boundary of gibbsite during calcination." Ceramics International. 46, pp. 12067-12072. https://doi.org/10.1016/j.ceramint.2020.01.248Catalyst-electrolyte Interactions in Aqueous Reline Solutions for Highly Selective Electrochemical CO2 Reduction
Garg, Sahil, Li, Mengran, Rufford, Thomas E., Ge, Lei, Rudolph, Victor, Knibbe, Ruth, Konarova, Muxina and Wang, Geoff G.X.. 2020. "Catalyst-electrolyte Interactions in Aqueous Reline Solutions for Highly Selective Electrochemical CO2 Reduction." ChemSusChem: chemistry and sustainability, energy and materials. 13 (2), pp. 304-311. https://doi.org/10.1002/cssc.201902433Enhanced thermoelectric properties of nanostructured n-type Bi2Te3 by suppressing Te vacancy through non-equilibrium fast reaction
Wang, Yuan, Liu, Wei-Di, Shi, XIao-Lei, Hong, Min, Wang, Li-Jun, Li, Meng, Wang, Hao, Zou, Jin and Chen, Zhi-Gang. 2020. "Enhanced thermoelectric properties of nanostructured n-type Bi2Te3 by suppressing Te vacancy through non-equilibrium fast reaction." Chemical Engineering Journal. 391. https://doi.org/10.1016/j.cej.2019.123513Development of a new calcium sulfoaluminate (synthetic ye'elimite) blended PII 52.5 cement
Zhang, Yu, Zhang, Zuhua, Shi, Chaoqi, Wang, Hao and Shen, Xiaodong. 2017. "Development of a new calcium sulfoaluminate (synthetic ye'elimite) blended PII 52.5 cement." Advances in Cement Research. 29 (9), pp. 373-386. https://doi.org/10.1680/jadcr.17.00027Accurate determination of the 'time-zero' of autogenous shrinkage in alkali-activated fly ash/slag system
Ma, Y., Yang, X., Hu, J., Zhang, Z. and Wang, H.. 2019. "Accurate determination of the 'time-zero' of autogenous shrinkage in alkali-activated fly ash/slag system." Composites Part B: Engineering. 177, pp. 1-8. https://doi.org/10.1016/j.compositesb.2019.107367Microstructure and wear characteristics of ATZ ceramic particle reinforced gray iron matrix surface composites
Ma, Xue, Li, Liang-feng, Zhang, Fan, Zhang, Zu-hua, Wang, Hao and Wang, En-ze. 2018. "Microstructure and wear characteristics of ATZ ceramic particle reinforced gray iron matrix surface composites." China Foundry. 15 (3), pp. 167-172. https://doi.org/10.1007/s41230-018-7211-6New selective dissolution process to quantify reaction extent and product stability in metakaolin-based geopolymers
Longhi, Marlon, Walkley, Brant, Rodriguez, Erich D, Kirchheim, Ana P, Zhang, Zuhua and Wang, Hao. 2019. "New selective dissolution process to quantify reaction extent and product stability in metakaolin-based geopolymers." Composites Part B: Engineering. 176 (1). https://doi.org/10.1016/j.compositesb.2019.107172Polylactide/hemp hurd biocomposites as sustainable 3D printing feedstock
Xiao, Xianglian, Chevali, Venkata S., Song, Pingan, He, Dongning and Wang, Hao. 2019. "Polylactide/hemp hurd biocomposites as sustainable 3D printing feedstock." Composites Science and Technology. 184, pp. 1-8. https://doi.org/10.1016/j.compscitech.2019.107887Efflorescence of alkali-activated cements (geopolymers) and the impacts on material structures: A critical analysis
Longhi, Marlon, Zhang, Zuhua, Rodriguez, Erich, Kirchheim, Ana and Wang, Hao. 2019. "Efflorescence of alkali-activated cements (geopolymers) and the impacts on material structures: A critical analysis." Frontiers in Materials. 6, pp. 1-13. https://doi.org/10.3389/fmats.2019.00089A review on mixture design methods for geopolymer concrete
Li, Ning, Shi, Caijun, Zhang, Zuhua, Wang, Hao and Liu, Yiwei. 2019. "A review on mixture design methods for geopolymer concrete." Composites Part B: Engineering. 178, pp. 1-14. https://doi.org/10.1016/j.compositesb.2019.107490Fine-Tuning the Coordinatively Unsaturated Metal Sites of Metal−Organic Frameworks by Plasma Engraving for Enhanced Electrocatalytic Activity
Jiang, Zongrui, Ge, Lei, Zhuang, Linzhou, Li, Mengran, Wang, Zhanke and Zhu, Zhonghua. 2019. "Fine-Tuning the Coordinatively Unsaturated Metal Sites of Metal−Organic Frameworks by Plasma Engraving for Enhanced Electrocatalytic Activity." ACS Applied Materials and Interfaces. 11 (47), pp. 44300-44307. https://doi.org/10.1021/acsami.9b15794A Surfactant‐Free and Scalable General Strategy for Synthesizing Ultrathin Two‐Dimensional Metal–Organic Framework Nanosheets for the Oxygen Evolution Reaction
Zhuang, Linzhou, Ge, Lei, Liu, Hongli, Jiang, Zongrui, Jia, Yi, Li, Zhiheng, Yang, Dongjiang, Hocking, Rosalie K., Li, Mengran, Zhang, Longzhou, Wang, Xing, Yao, Xiangdong and Zhu, Zhonghua. 2019. "A Surfactant‐Free and Scalable General Strategy for Synthesizing Ultrathin Two‐Dimensional Metal–Organic Framework Nanosheets for the Oxygen Evolution Reaction." Angewandte Chemie. 58, pp. 13565-13572. https://doi.org/10.1002/anie.201907600Metal-free graphene/boron nitride heterointerface for CO2 reduction: Surface curvature controls catalytic activity and selectivity
Mao, Xin, Wijethunge, Dimuthu, Zhang, Lei, Wang, Sufan, Yan, Cheng, Zhu, Zhonghua and Du, Aijun. 2020. "Metal-free graphene/boron nitride heterointerface for CO2 reduction: Surface curvature controls catalytic activity and selectivity." Ecomat. 2 (1). https://doi.org/10.1002/eom2.12013Computational screening of MN 4 (M= Ti–Cu) based metal organic frameworks for CO 2 reduction using the d-band centre as a descriptor
Mao, Mao, Tang, Cheng, He, Tianwei, Wijethunge, Dimuthu, Yan, Cheng, Zhu, Zhonghua and Du, Aijun. 2020. "Computational screening of MN 4 (M= Ti–Cu) based metal organic frameworks for CO 2 reduction using the d-band centre as a descriptor." Nanoscale. 12 (10), pp. 6188-6194. https://doi.org/10.1039/C9NR09529BWater absorption and chloride diffusivity of concrete under the coupling effect of uniaxial compressive load and freeze-thaw cycles
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Fu, H. M., Qiu, D., Zhang, M. X., Wang, H., Kelly, P. M. and Taylor, J. A.. 2008. "The development of a new grain refiner for magnesium alloys using the edge-to-edge model." Journal of Alloys and Compounds. 456 (1-2), pp. 390-394. https://doi.org/10.1016/j.jallcom.2007.02.076Cu-based bulk amorphous alloy with larger glass-forming ability and supercooled liquid region
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Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of Carbon Nanotubes and Metal Catalysts on Hydrogen Storage in Magnesium Nanocomposites." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498. https://doi.org/10.1166/jnn.2006.098In situ TiB-reinforced cu-based bulk metallic glass composites
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "In situ TiB-reinforced cu-based bulk metallic glass composites." Scripta Materialia. 54 (11), pp. 1961-1966. https://doi.org/10.1016/j.scriptamat.2006.01.048Numerical simulation of dendrite growth during solidification
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Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2006. "In-situ Cu-based bulk metallic glass composite." International Journal of Modern Physics B. 20 (25-27), pp. 3963-3968. https://doi.org/10.1142/S0217979206040696The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
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Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "Tungsten fibre reinforced Zr-based bulk metallic glass composites ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2007. "Tungsten fibre reinforced Zr-based bulk metallic glass composites." Materials and Manufacturing Processes. 22 (5-6), pp. 687-691. https://doi.org/10.1080/10426910701384922Semisolid structure simulation in controlled nucleation process
Wang, H. and Yao, X. D.. 2006. "Semisolid structure simulation in controlled nucleation process." Solid State Phenomena. 116-117, pp. 614-617. https://doi.org/10.4028/www.scientific.net/SSP.116-117.614The effect of initial microstructure of A356 alloys on the mechanical behavior in the semisolid state
Ning, Zhiliang, Wang, Hao and Sun, Jianfei. 2006. "The effect of initial microstructure of A356 alloys on the mechanical behavior in the semisolid state." Solid State Phenomena. 116-117, pp. 449-452. https://doi.org/10.4028/www.scientific.net/SSP.116-117.449Semisolid casting of automotive component: water pump lid
Wang, Hao and Xu, Jun. 2006. "Semisolid casting of automotive component: water pump lid." Solid State Phenomena. 116-117, pp. 88-91. https://doi.org/10.4028/www.scientific.net/SSP.116-117.88The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ
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Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Canning, John. 2010. "Effects of the self distortions of embedded FBG sensors on spectral response due to torsional and combined loads." 3rd Asia-Pacific Workshop on Structural Health Monitoring (APWSHM 2010). Tokyo, Japan 30 Nov - 02 Dec 2010 Tokyo, Japan.Natural fibre composites with epoxidized vegetable oil (EVO) resins: a review
Manthey, N. W., Cardona, F., Aravinthan, T., Wang, H. and Cooney, T.. 2010. "Natural fibre composites with epoxidized vegetable oil (EVO) resins: a review." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Magnesium and magnesium alloys as degradable metallic biomaterials
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Ning, Zhiliang, Wu, Peilian, Wang, Hao, Cao, Fuyang and Sun, Jianfei. 2007. "Effect of pouring temperature on thixotropic microstructure formation of AZ91." Rare Metals. 26 (S1), pp. 180-184.Anomalous grain coarsening behaviour observed in grain-refined aluminium alloy cast using low superheat
Taylor, J. A., Wang, H., StJohn, D. H. and Bainbridge, I. F.. 2001. "Anomalous grain coarsening behaviour observed in grain-refined aluminium alloy cast using low superheat." Anjier, Joseph L. (ed.) 130th TMS Annual MeetingLight Metals 2001. New Orleans, Louisanna 11 - 15 Feb 2001 Warrendale, PA. United States.Semisolid microstructural evolution of AlSi7Mg during partial remelting
Wang, Hao, Davidson, C. J. and StJohn, David H.. 2004. "Semisolid microstructural evolution of AlSi7Mg during partial remelting." Materials Science and Engineering A: Structural Materials: Properties, Microstructure and Processing. 368 (1-2), pp. 159-167. https://doi.org/10.1016/j.msea.2003.10.305Biocorrosion behaviour of magnesium alloys under pseudo-physiological conditions
Wang, Hao, Zhang, M. X., Shi, Z. M. and Yang, Ke. 2006. "Biocorrosion behaviour of magnesium alloys under pseudo-physiological conditions." Tissue Engineering. 12 (4), pp. 1067-1067.Facile one-pot synthesis of MOF supported gold pseudo-single-atom catalysts for hydrogenation reactions
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