Dynamic Nanoconfinement Enabled Highly Stretchable and Supratough Polymeric Materials with Desirable Healability and Biocompatibility
Article
Liu, Lei, Zhu, Menghe, Xu, Xiaodong, Ma, Zhewen, Jiang, Zhen, Pich, Andrij, Wang, Hao, Song, Pingan and Li, X.. 2021. "Dynamic Nanoconfinement Enabled Highly Stretchable and Supratough Polymeric Materials with Desirable Healability
and Biocompatibility." Advanced Materials. 33 (51), pp. 1-11. https://doi.org/10.1002/adma.202105829
| Article Title | Dynamic Nanoconfinement Enabled Highly Stretchable and Supratough Polymeric Materials with Desirable Healability |
|---|---|
| ERA Journal ID | 4865 |
| Article Category | Article |
| Authors | Liu, Lei (Author), Zhu, Menghe (Author), Xu, Xiaodong (Author), Ma, Zhewen (Author), Jiang, Zhen (Author), Pich, Andrij (Author), Wang, Hao (Author), Song, Pingan (Author) and Li, X. |
| Journal Title | Advanced Materials |
| Journal Citation | 33 (51), pp. 1-11 |
| Article Number | 2105829 |
| Number of Pages | 11 |
| Year | 2021 |
| Publisher | John Wiley & Sons |
| Place of Publication | Germany |
| ISSN | 0935-9648 |
| 1521-4095 | |
| Digital Object Identifier (DOI) | https://doi.org/10.1002/adma.202105829 |
| Web Address (URL) | https://onlinelibrary.wiley.com/doi/full/10.1002/adma.202105829 |
| Abstract | Lightweight polymeric materials are highly attractive platforms for many potential industrial applications in aerospace, soft robots, and biological engineering fields. For these real-world applications, it is vital for them to exhibit a desirable combination of great toughness, large ductility, and high strength together with desired healability and biocompatibility. However, existing material design strategies usually fail to achieve such a performance portfolio owing to their different and even mutually exclusive governing mechanisms. To overcome these hurdles, herein, for the first time a dynamic hydrogen-bonded nanoconfinement concept is proposed, and the design of highly stretchable and supratough biocompatible poly(vinyl alcohol) (PVA) with well-dispersed dynamic nanoconfinement phases induced by hydrogen-bond (H-bond) crosslinking is demonstrated. Because of H-bond crosslinking and dynamic nanoconfinement, the as-prepared PVA nanocomposite film exhibits a world-record toughness of 425 ± 31 MJ m−3 in combination with a tensile strength of 98 MPa and a large break strain of 550%, representing the best of its kind and even outperforming most natural and artificial materials. In addition, the final polymer exhibits a good self-healing ability and biocompatibility. This work affords new opportunities for creating mechanically robust, healable, and biocompatible polymeric materials, which hold great promise for applications, such as soft robots and artificial ligaments. |
| Keywords | biocompatibility; healability; nanoconfinement; supratough polymers |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Institution of Origin | University of Southern Queensland |
| Byline Affiliations | Zhejiang A & F University, China |
| Centre for Future Materials | |
| Leibniz Institute for Interactive Materials, Germany | |
| DWI Leibniz Institute for Interactive Materials, Germany |
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Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498.In situ TiB-reinforced cu-based bulk metallic glass composites
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Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2006. "In-situ Cu-based bulk metallic glass composite." International Journal of Modern Physics B. 20 (25-27), pp. 3963-3968. https://doi.org/10.1142/S0217979206040696The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
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Wang, Hao. 2006. "In-situ Si/Al composite produced by semisolid metal processing ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
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Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2007. "Tungsten fibre reinforced Zr-based bulk metallic glass composites." Materials and Manufacturing Processes. 22 (5-6), pp. 687-691. https://doi.org/10.1080/10426910701384922The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ
Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Aravinthan, Thiru. 2010. "The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Sustainable materials research at USQ
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Ning, Z. L., Wang, H., Liu, H. H., Cao, F. Y., Wang, S. T. and Sun, J. F.. 2010. "Effects of Nd on microstructures and properties at the elevated temperature of a Mg-0.3Zn-0.32Zr alloy." Materials and Design. 31 (9), pp. 4438-4444. https://doi.org/10.1016/j.matdes.2010.04.021The role of casting temperature in preparation of bulk metallic glasses
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Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2007. "A practical thermodynamic method to calculate the best glass-forming composition for bulk metallic glasses." International Journal of Nonlinear Sciences and Numerical Simulation. 8 (2), pp. 171-178.Effect of cooling conditions on grain size of AZ91 alloy
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Song, Pingan, Zhu, Yan, Tong, Lifang and Fang, Zhengping. 2008. "C60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network." Nanotechnology. 19 (22). https://doi.org/10.1088/0957-4484/19/22/225707Polypropylene/clay nanocomposites prepared by in situ grafting–melt intercalation with a novel co-intercalating monomer
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Fang, Zhengping, Song, Pingan, Tong, Lifang and Guo, Zhenghong. 2008. "Thermal degradation and flame retardancy of polypropylene/C60 nanocomposites." Thermochimica Acta. 473 (1), pp. 106-108. https://doi.org/10.1016/j.tca.2008.04.019Effects of metal chelates on a novel oligomeric intumescent flame retardant system for polypropylene
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Wang, Hao, Zhang, M. X., Shi, Z. M. and Yang, Ke. 2006. "Biocorrosion behaviour of magnesium alloys under pseudo-physiological conditions." Tissue Engineering. 12 (4), pp. 1067-1067.Semisolid structure simulation in controlled nucleation process
Wang, H. and Yao, X. D.. 2006. "Semisolid structure simulation in controlled nucleation process." Solid State Phenomena. 116-117, pp. 614-617.The effect of initial microstructure of A356 alloys on the mechanical behavior in the semisolid state
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