Realizing simultaneous improvements in mechanical strength, flame retardancy and smoke suppression of ABS nanocomposites from multifunctional graphene
Article
Huang, Guobo, Huo, Siqi, Xu, Xiaodong, Chen, Wei, Jin, Yanxian, Li, Rongrong, Song, Pingan and Wang, Hao. 2019. "Realizing simultaneous improvements in mechanical strength, flame retardancy and smoke suppression of ABS nanocomposites from multifunctional graphene." Composites Part B: Engineering. 177, pp. 1-10. https://doi.org/10.1016/j.compositesb.2019.107377
| Article Title | Realizing simultaneous improvements in mechanical strength, flame retardancy and smoke suppression of ABS nanocomposites from multifunctional graphene |
|---|---|
| ERA Journal ID | 4883 |
| Article Category | Article |
| Authors | Huang, Guobo (Author), Huo, Siqi (Author), Xu, Xiaodong (Author), Chen, Wei (Author), Jin, Yanxian (Author), Li, Rongrong (Author), Song, Pingan (Author) and Wang, Hao |
| Journal Title | Composites Part B: Engineering |
| Journal Citation | 177, pp. 1-10 |
| Article Number | 107377 |
| Number of Pages | 10 |
| Year | 2019 |
| Publisher | Elsevier |
| Place of Publication | United Kingdom |
| ISSN | 1359-8368 |
| Digital Object Identifier (DOI) | https://doi.org/10.1016/j.compositesb.2019.107377 |
| Web Address (URL) | https://www.sciencedirect.com/science/article/abs/pii/S1359836819331117 |
| Abstract | Acrylonitrile-butadiene-styrene (ABS), as one of the most widely used engineering plastics, suffers from the problem of serious flammability and low mechanical strength. To address such an intractable challenge, herein, we report the design of a graphene-based multifunctional additive (Sb-Mo/Br-rGO) via the bromination followed by precipitating antimony molybdenum. The surface functionalization enables Sb-Mo/Br-rGO to homogeneously disperse within the ABS matrix through facile melt-blending. The incorporation of 5 wt% Sb-Mo/Br-rGO leads to a 31% increase in tensile strength and 73% increase in elastic modulus relative to the ABS bulk. In addition to significant enhancement in thermal stability, the inclusion of 5 wt% Sb-Mo/Br-rGO significantly delays the time to ignition of ABS by 12 s, and noticeably reduces the peak heat release rate (PHRR) and total smoke production (TSP) by 45% and 54%, respectively. Such improved performance portfolio is primarily because the mechanical reinforcing and thermal barrier effect of graphene nanosheets, the flame retardant effect of bromine/antimony, and the smoke suppression action of antimony molybdenum. This work provides an innovative methodology for the design of multifunctional additives to create high-performance polymeric materials with high strength and low flammability, thus contributing to improving the quality of life. |
| Keywords | Acrylonitrile-butadiene-styrene (ABS); GrapheneFlame retardancy; Smoke suppression; Mechanical property |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401807. Nanomaterials | |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | Taizhou University, China |
| Centre for Future Materials | |
| Zhejiang A & F University, China | |
| Institution of Origin | University of Southern Queensland |
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Wang, Hao and Ning, Zhiliang. 2007. "Magnesium thixotropic structure produced by controlled nucleation method ." Tezhong Zhuzao Ji Youse Hejin (Special Casting and Nonferrous Alloys).In-situ Si/Al composite produced by semisolid metal processing
Wang, Hao. 2007. "In-situ Si/Al composite produced by semisolid metal processing." Materials and Manufacturing Processes. 22 (5-6), pp. 696-699. https://doi.org/10.1080/10426910701384963The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31
Wang, H., Estrin, Y., Fu, H. M., Song, G. L. and Zuberova, Z.. 2007. "The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31." Advanced Engineering Materials. 9 (11), pp. 967-972. https://doi.org/10.1002/adem.200700200Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite
Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498.In situ TiB-reinforced cu-based bulk metallic glass composites
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "In situ TiB-reinforced cu-based bulk metallic glass composites." Scripta Materialia. 54 (11), pp. 1961-1966. https://doi.org/10.1016/j.scriptamat.2006.01.048In-situ Cu-based bulk metallic glass composite
Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2006. "In-situ Cu-based bulk metallic glass composite." International Journal of Modern Physics B. 20 (25-27), pp. 3963-3968. https://doi.org/10.1142/S0217979206040696The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
Yao, X. and Wang, H.. 2006. "Modeling of semisolid structure formation in controlled nucleation method ." International Journal of Modern Physics B. 20 (25-27), pp. 4123-4128. https://doi.org/10.1142/S0217979206040969In-situ Si/Al composite produced by semisolid metal processing
Wang, Hao. 2006. "In-situ Si/Al composite produced by semisolid metal processing ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "Tungsten fibre reinforced Zr-based bulk metallic glass composites ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2007. "Tungsten fibre reinforced Zr-based bulk metallic glass composites." Materials and Manufacturing Processes. 22 (5-6), pp. 687-691. https://doi.org/10.1080/10426910701384922The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ
Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Aravinthan, Thiru. 2010. "The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Sustainable materials research at USQ
Wang, Hao. 2010. "Sustainable materials research at USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia .Influence of casting temperature on microstructures and mechanical properties of Cu50Zr45.5Ti2.5Y2 metallic glass prepared using copper mold casting [+ Erratum]
Zhu, Zhengwang, Zhang, Haifeng, Wang, Hao, Ding, Bingzhe, Hu, Zhuang-Qi and Huang, Han. 2009. "Influence of casting temperature on microstructures and mechanical properties of Cu50Zr45.5Ti2.5Y2 metallic glass prepared using copper mold casting [+ Erratum]." Journal of Materials Research. 24 (10), pp. 3108-3115. https://doi.org/10.1557/jmr.2009.0373Deformation behavior of semisolid A356 alloy prepared by low temperature pouring
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Kabir, Mohammad Mazedul, Islam, Md Mainul and Wang, Hao. 2010. "Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites." 1st International Conference on Mechanical, Industrial and Energy Engineering (ICMIEE 2010) . Khulna, Bangladesh 23 - 24 Dec 2010 Khulna, Bangladesh.An investigation of spectral response of embedded Fibre Bragg Grating (FBG) sensors in a hollow composite cylindrical beam under pure torsion and combined loading
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Manthey, N. W., Cardona, F., Aravinthan, T., Wang, H. and Cooney, T.. 2010. "Natural fibre composites with epoxidized vegetable oil (EVO) resins: a review." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Magnesium and magnesium alloys as degradable metallic biomaterials
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Ren, Yibin, Huang, Jingjing, Yang, Ke, Zhang, Bingchun, Yao, Zhiming and Wang, Hao. 2005. "Study of bio-corrosion of pure magnesium." Jinshu Xuebao. 41 (11), pp. 1228-1232.Present status and future trends in production of semisolid materials
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Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2010. "Effects of corona discharge on the surface structure, morphology and properties of multi-walled carbon nanotubes." Applied Surface Science. 256 (21), pp. 6447-6453. https://doi.org/10.1016/j.apsusc.2010.04.033Biodegradable aliphatic/aromatic copolymers based on terephthalic acid and poly(L-lactic acid): Synthesis, characterization and hydrolytic degradation
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Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2010. "Functionalization of carbon nanotubes by corona-discharge induced graft polymerization for the reinforcement of epoxy nanocomposites." Plasma Processes and Polymers. 7 (9), pp. 785-793. https://doi.org/10.1002/ppap.201000019Thermal degradation and flammability properties of HDPE/EVA/C60 nanocomposites
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Fu, Shenyuan, Song, Pingan, Yang, Haitang, Jin, Yongming, Lu, Fengzhu, Ye, Jiewang and Wu, Qiang. 2010. "Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites." Journal of Materials Science. 45 (13), pp. 3520-3528. https://doi.org/10.1007/s10853-010-4394-7Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol
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