Functionalizing MXene towards highly stretchable, ultratough, fatigue- and fire-resistant polymer nanocomposites
Article
Liu, Lei, Zhu, Menghe, Shi, Yongqian, Xu, Xiaodong, Ma, Zhewen, Yu, Bin, Fu, Shenyuan, Huang, Guobo, Wang, Hao and Song, Pingan. 2021. "Functionalizing MXene towards highly stretchable, ultratough, fatigue- and fire-resistant polymer nanocomposites." Chemical Engineering Journal. 424, pp. 1-13. https://doi.org/10.1016/j.cej.2021.130338
| Article Title | Functionalizing MXene towards highly stretchable, ultratough, fatigue- and fire-resistant polymer nanocomposites |
|---|---|
| ERA Journal ID | 3854 |
| Article Category | Article |
| Authors | Liu, Lei (Author), Zhu, Menghe (Author), Shi, Yongqian (Author), Xu, Xiaodong (Author), Ma, Zhewen (Author), Yu, Bin (Author), Fu, Shenyuan (Author), Huang, Guobo (Author), Wang, Hao (Author) and Song, Pingan (Author) |
| Journal Title | Chemical Engineering Journal |
| Journal Citation | 424, pp. 1-13 |
| Article Number | 130338 |
| Number of Pages | 13 |
| Year | 2021 |
| Publisher | Elsevier |
| Place of Publication | Netherlands |
| ISSN | 1385-8947 |
| 1873-3212 | |
| Digital Object Identifier (DOI) | https://doi.org/10.1016/j.cej.2021.130338 |
| Web Address (URL) | https://www.sciencedirect.com/science/article/pii/S1385894721019240 |
| Abstract | Thermoplastic polyurethane (TPU) features many important industrial applications, but intrinsic flammability extremely impedes its practical applications. Current fire-retardant strategies often lead to improved flame retardancy but reduced mechanical properties (strength, ductility, and toughness). Hence, to date it has been unsuccessful to design advanced TPU materials that are strong, stretchable, tough, fatigue-and fire-resistant to meet increasing performance portfolio requirements. Here, we report a hybridized fire retardant (Zr-MXene) by in situ facilely loading zirconium amino-tris-(methylenephosphonate) (Zr-AMP) onto the titanium carbide (MXene) surface. Our results show that with 1 wt% of Zr-MXene, the resultant TPU nanocomposites demonstrate a record break strain (2060%) and toughness (316 MJ/m3) to date, in addition to increased tensile strength by 43.4% and improved fatigue resistance relative to the TPU matrix, because of favorable interfacial hydrogen-bonding. Moreover, the resultant TPU material exhibit significantly reduced flammability as a result of the combined physical barrier, catalytical carbonization and diluting effects of Zr-MXene. This work provides a promising strategy for the creation of multifunctional MXene and its polymeric nanocomposites, which hold great promise for many industrial applications. |
| Keywords | MXene; Thermoplastic polyurethane; Mechanical property; Flame retardancy; Smoke suppression |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | Zhejiang A & F University, China |
| Tongji University, China | |
| Fuzhou University, China | |
| University of Science and Technology of China, China | |
| Taizhou University, China | |
| Centre for Future Materials | |
| Institution of Origin | University of Southern Queensland |
| Funding source | Australian Research Council (ARC) Grant ID DP190102992 |
| Funding source | Australian Research Council (ARC) Grant ID FT190100188 |
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Kahandawa, G. C., Epaarachchi, J. A., Wang, H., Followell, D. and Birt, P.. 2013. "Use of fixed wavelength Fibre-Bragg Grating (FBG) filters to capture time domain data from the distorted spectrum of an embedded FBG sensor to estimate strain with an artificial neural network." Sensors and Actuators A: Physical. 194, pp. 1-7. https://doi.org/10.1016/j.sna.2012.12.028Quantitative kinetic and structural analysis of geopolymers. Part 1. The activation of metakaolin with sodium hydroxide
Zhang, Zuhua, Wang, Hao, Provis, John L., Bullen, Frank, Reid, Andrew and Zhu, Yingcan. 2012. "Quantitative kinetic and structural analysis of geopolymers. Part 1. The activation of metakaolin with sodium hydroxide." Thermochimica Acta. 539, pp. 23-33. https://doi.org/10.1016/j.tca.2012.03.021Numerical simulation of porous structure in foam concrete on thermal insulation property
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Ho, Mei-po, Wang, Hao, Lau, Kin-tak, Lee, Joong-hee and Hui, David. 2012. "Interfacial bonding and degumming effects on silk fibre/polymer biocomposites ." Composites Part B: Engineering. 43 (7), pp. 2801-2812. https://doi.org/10.1016/j.compositesb.2012.04.042Potential application of geopolymers as protection coatings for marine concrete III. Field experiment
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Ho, Mei-Po, Lau, Kin-tak, Wang, Hao and Bhattacharyya, Debes. 2011. "Mechanical properties of an injected silk fibre reinforced PLA composite." Bhattacharyya, D., Lin, R. J. T. and Srivatsan, T. S. (ed.) 19th International Symposium on Processing and Fabrication of Advanced Materials (PFAM XIX). Auckland, New Zealand 14 - 17 Jan 2011 Auckland, New Zealand.Flexural strength of sandwich panel with lignocellulosic composites intermediate layer: a statistic approach
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Hua, Fuan, Zhang, Chaoyi, Li, Qiang, Yu, Baoyi, Liu, Weihua, Li, Runxia, Xie, Shuisheng, Huang, Guojie, Cheng, Lei, Fu, Yao and Wang, Hao. 2011. "Numerical simulation of rolling process and microstructure evolution of AM50 Mg alloy during hot rolling process ." Advanced Materials Research. 291-294, pp. 449-454. https://doi.org/10.4028/www.scientific.net/AMR.291-294.449Deformation behaviour of aluminum alloy A356 in semisolid state
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Zhu, Z. W., Zhang, H. F., Wang, H., Ding, B. Z. and Hu, Z. Q.. 2008. "Influence of casting temperature on the thermal stability of Cu- and Zr-based metallic glasses: theoretical analysis and experiments." Journal of Materials Research. 23 (10), pp. 2714-2719. https://doi.org/10.1557/jmr.2008.0335Solidification microstructure modelling using cellular automaton method
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Fu, H. M., Qiu, D., Zhang, M. X., Wang, H., Kelly, P. M. and Taylor, J. A.. 2008. "The development of a new grain refiner for magnesium alloys using the edge-to-edge model." Journal of Alloys and Compounds. 456 (1-2), pp. 390-394. https://doi.org/10.1016/j.jallcom.2007.02.076Cu-based bulk amorphous alloy with larger glass-forming ability and supercooled liquid region
Fu, H. M., Zhang, H. F., Wang, H. and Hu, Z. Q.. 2008. "Cu-based bulk amorphous alloy with larger glass-forming ability and supercooled liquid region." Journal of Alloys and Compounds. 458 (1-2), pp. 390-393. https://doi.org/10.1016/j.jallcom.2007.03.114Study of biodegradation of pure magnesium
Ren, Yibin, Wang, Hao, Huang, Jingjing, Zhang, Bingchun and Yang, Ke. 2007. "Study of biodegradation of pure magnesium." Kim, Young-Ha, Cho, Chong-Su, Kang, Inn-Kyu, Kim, Suk Young and Kwon, Oh Hyeong (ed.) ASBM7: 7th Asian Symposium on Biomedical Materials. Jeju, Korea 20 - 23 Aug 2006 Switzerland. https://doi.org/10.4028/www.scientific.net/KEM.342-343.601The use of simulated games in an undergraduate course manufacturing processes
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Fu, H. M., Zhang, H. F., Wang, Hao, Zhang, Qingsheng and Hu, Z. Q.. 2005. "Synthesis and mechanical properties of Cu-based bulk metallic glass composites containing in-situ TiC particles." Scripta Materialia. 52 (7), pp. 669-673. https://doi.org/10.1016/j.scriptamat.2004.10.031Preface to futures in mechanics of structures and materials conference. ACMSM20
Aravinthan, Thiru, Karunasena, Warna (Karu) and Wang, Hao. 2009. "Preface to futures in mechanics of structures and materials conference. ACMSM20." Aravinthan, Thiru, Karunasena, Warna (Karu) and Wang, Hao (ed.) 20th Australasian Conference on the Mechanics of Structures and Materials (ACMSM20). Toowoomba, Australia 02 - 05 Dec 2008 London, United Kingdom.Magnesium thixotropic structure produced by controlled nucleation method
Wang, Hao and Ning, Zhiliang. 2007. "Magnesium thixotropic structure produced by controlled nucleation method ." Tezhong Zhuzao Ji Youse Hejin (Special Casting and Nonferrous Alloys).In-situ Si/Al composite produced by semisolid metal processing
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Wang, H., Estrin, Y., Fu, H. M., Song, G. L. and Zuberova, Z.. 2007. "The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31." Advanced Engineering Materials. 9 (11), pp. 967-972. https://doi.org/10.1002/adem.200700200Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite
Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498.In situ TiB-reinforced cu-based bulk metallic glass composites
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Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
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Li, Qiang, Yu, Baoyi, Zhang, Huawen, Li, Runxia, Wang, Feng, Xie, Shuisheng, Huang, Guojie and Wang, Hao. 2010. "Cellular automaton modeling of semisolid microstructure formation." China Foundry. 7 (2), pp. 143-148.Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites
Kabir, Mohammad Mazedul, Islam, Md Mainul and Wang, Hao. 2010. "Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites." 1st International Conference on Mechanical, Industrial and Energy Engineering (ICMIEE 2010) . Khulna, Bangladesh 23 - 24 Dec 2010 Khulna, Bangladesh.An investigation of spectral response of embedded Fibre Bragg Grating (FBG) sensors in a hollow composite cylindrical beam under pure torsion and combined loading
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Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Canning, John. 2010. "Effects of the self distortions of embedded FBG sensors on spectral response due to torsional and combined loads." 3rd Asia-Pacific Workshop on Structural Health Monitoring (APWSHM 2010). Tokyo, Japan 30 Nov - 02 Dec 2010 Tokyo, Japan.Natural fibre composites with epoxidized vegetable oil (EVO) resins: a review
Manthey, N. W., Cardona, F., Aravinthan, T., Wang, H. and Cooney, T.. 2010. "Natural fibre composites with epoxidized vegetable oil (EVO) resins: a review." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Magnesium and magnesium alloys as degradable metallic biomaterials
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Ren, Yibin, Huang, Jingjing, Yang, Ke, Zhang, Bingchun, Yao, Zhiming and Wang, Hao. 2005. "Study of bio-corrosion of pure magnesium." Jinshu Xuebao. 41 (11), pp. 1228-1232.Present status and future trends in production of semisolid materials
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Ouyang, L. Z., Wang, Hao, Zhu, M., Zou, Jin and Chung, C. Y.. 2004. "Microstructure of MmM5/Mg multi-layer hydrogen storage films prepared by magnetron sputtering." Microscopy Research and Technique. 64 (4), pp. 323-329. https://doi.org/10.1002/jemt.20089Crystallization behavior of (Cu60Zr30Ti10)99Sn1 bulk metallic glass
Wang, Hao, Song, Xiaoping, Yao, Xiangdong, Zhang, Haifeng and Hu, Zhuangqui. 2005. "Crystallization behavior of (Cu60Zr30Ti10)99Sn1 bulk metallic glass." Journal of Materials Science and Technology. 21 (1 (Supplement)), pp. 51-53.Effects of corona discharge on the surface structure, morphology and properties of multi-walled carbon nanotubes
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Wang, Bing-tao, Zhang, Yan, Song, Pingan, Guo, Zhenghong, Cheng, Jie and Fang, Zhengping. 2010. "Biodegradable aliphatic/aromatic copolymers based on terephthalic acid and poly(L-lactic acid): Synthesis, characterization and hydrolytic degradation." Chinese Journal of Polymer Science. 28 (1), pp. 405-415. https://doi.org/10.1007/s10118-010-9032-yFunctionalization of carbon nanotubes by corona-discharge induced graft polymerization for the reinforcement of epoxy nanocomposites
Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2010. "Functionalization of carbon nanotubes by corona-discharge induced graft polymerization for the reinforcement of epoxy nanocomposites." Plasma Processes and Polymers. 7 (9), pp. 785-793. https://doi.org/10.1002/ppap.201000019Thermal degradation and flammability properties of HDPE/EVA/C60 nanocomposites
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Fu, Shenyuan, Song, Pingan, Yang, Haitang, Jin, Yongming, Lu, Fengzhu, Ye, Jiewang and Wu, Qiang. 2010. "Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites." Journal of Materials Science. 45 (13), pp. 3520-3528. https://doi.org/10.1007/s10853-010-4394-7Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol
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