Grafting Lignin with Bioderived Polyacrylates for Low-Cost, Ductile, and Fully Biobased Poly(lactic acid) Composite
Article
Sun, Yiqi, Ma, Zhewen, Xu, Xiaodong, Liu, Xiaohuan, Liu, Lina, Huang, Guobo, Liu, Lei, Wang, Hao and Song, Pingan. 2020. "Grafting Lignin with Bioderived Polyacrylates for Low-Cost, Ductile, and Fully Biobased Poly(lactic acid) Composite." ACS Sustainable Chemistry and Engineering. 8 (5), pp. 2267-2276. https://doi.org/10.1021/acssuschemeng.9b06593
| Article Title | Grafting Lignin with Bioderived Polyacrylates for Low-Cost, Ductile, and Fully Biobased Poly(lactic acid) Composite |
|---|---|
| ERA Journal ID | 200101 |
| Article Category | Article |
| Authors | Sun, Yiqi (Author), Ma, Zhewen (Author), Xu, Xiaodong (Author), Liu, Xiaohuan (Author), Liu, Lina (Author), Huang, Guobo (Author), Liu, Lei (Author), Wang, Hao (Author) and Song, Pingan (Author) |
| Journal Title | ACS Sustainable Chemistry and Engineering |
| Journal Citation | 8 (5), pp. 2267-2276 |
| Number of Pages | 10 |
| Year | 2020 |
| Publisher | American Chemical Society |
| Place of Publication | United States |
| ISSN | 2168-0485 |
| Digital Object Identifier (DOI) | https://doi.org/10.1021/acssuschemeng.9b06593 |
| Web Address (URL) | https://pubs.acs.org/doi/10.1021/acssuschemeng.9b06593 |
| Abstract | It has been always attractive to design low-cost, ductile, and fully biobased polylactic acid (PLA) composites based on industrial waste lignin for promoting its practical applications in the industry. Unfortunately, existing material strategies often lead to poor processability and low ductility because of weak interfaces between lignin and PLA. Herein, we report a fully biobased functionalized lignin (Lig-g-P(LMA-co-THFMA, or Mlignin) by chemically grafting two bioderived monomers, lauryl methacrylate (LMA), and tetrahydrofurfuryl methacrylate (THFMA) via free-radical polymerization. Mlignin exhibits moderately lower melt viscosity and improved formability with PLA as compared with pristine lignin due to better interfacial combability. Because of improved interfacial adhesion, Mlignin is capable of uniformly dispersing within the PLA matrix in a submicron phase size, leading to a “sea-island” structure. As a result, the addition of 20 wt % Mlignin increases the ductility by 16 folds (from 12 to 204%) and the toughness by ∼11 folds from 4.4 to 54.6 MJ m–3 relative to the PLA matrix. Meanwhile, the PLA/20% Mlignin composite retains a tensile strength of 40.9 MPa. Such largely enhanced ductility and toughness of PLA is mainly attributed to the deformation of Mlignin that can dissipate the fracture energy during the tension process. This work not only offers a simple route to converting industrial waste lignin into value-added biobased fillers for polymers and but also provides a new approach for developing low-cost, ductile, and fully sustainable PLA to further its industrial applications. |
| Keywords | poly(lactic acid); lignin; chemical graft; toughness; ductility |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | Zhejiang A & F University, China |
| Taizhou University, China | |
| Centre for Future Materials | |
| Institution of Origin | University of Southern Queensland |
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Zhuang, Xiao Yu, Chen, Liang, Komarneni, Sridhar, Zhou, Chun Hui, Tong, Dong Shen, Yang, Hui Min, Yu, Wei Hua and Wang, Hao. 2016. "Fly ash-based geopolymer: clean production, properties and applications." Journal of Cleaner Production. 125, pp. 253-267. https://doi.org/10.1016/j.jclepro.2016.03.019Conversion of local industrial wastes into greener cement through geopolymer technology: a case study of high-magnesium nickel slag
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Hua, Fuan, Zhang, Chaoyi, Li, Qiang, Yu, Baoyi, Liu, Weihua, Li, Runxia, Xie, Shuisheng, Huang, Guojie, Cheng, Lei, Fu, Yao and Wang, Hao. 2011. "Numerical simulation of rolling process and microstructure evolution of AM50 Mg alloy during hot rolling process ." Advanced Materials Research. 291-294, pp. 449-454. https://doi.org/10.4028/www.scientific.net/AMR.291-294.449Deformation behaviour of aluminum alloy A356 in semisolid state
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Zhu, Z. W., Zhang, H. F., Wang, H., Ding, B. Z. and Hu, Z. Q.. 2008. "Influence of casting temperature on the thermal stability of Cu- and Zr-based metallic glasses: theoretical analysis and experiments." Journal of Materials Research. 23 (10), pp. 2714-2719. https://doi.org/10.1557/jmr.2008.0335Solidification microstructure modelling using cellular automaton method
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Fu, H. M., Qiu, D., Zhang, M. X., Wang, H., Kelly, P. M. and Taylor, J. A.. 2008. "The development of a new grain refiner for magnesium alloys using the edge-to-edge model." Journal of Alloys and Compounds. 456 (1-2), pp. 390-394. https://doi.org/10.1016/j.jallcom.2007.02.076Cu-based bulk amorphous alloy with larger glass-forming ability and supercooled liquid region
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Ren, Yibin, Wang, Hao, Huang, Jingjing, Zhang, Bingchun and Yang, Ke. 2007. "Study of biodegradation of pure magnesium." Kim, Young-Ha, Cho, Chong-Su, Kang, Inn-Kyu, Kim, Suk Young and Kwon, Oh Hyeong (ed.) ASBM7: 7th Asian Symposium on Biomedical Materials. Jeju, Korea 20 - 23 Aug 2006 Switzerland. https://doi.org/10.4028/www.scientific.net/KEM.342-343.601The use of simulated games in an undergraduate course manufacturing processes
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Yao, Xiangdong, Wang, Hao, He, B. and Zhou, X.. 2005. "Modeling of columnar-to-equiaxed transition in solidified Al-Si alloys." Zhong, Z., Saka, H., Kim, T. H., Holm, E. A., Han, Y. and Xie, X. (ed.) 5th Pacific Rim International Conference on Advanced Materials and Processing (PRICM 5). Beijing, China 02 - 05 Nov 2004 Zurich, Switzerland. Scientific.Net. https://doi.org/10.4028/www.scientific.net/MSF.475-479.3141Formation and mechanical properties of Mg65Cu25Er10 and Mg65Cu15Ag10Er10 bulk amorphous alloys
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Fu, H. M., Zhang, H. F., Wang, Hao, Zhang, Qingsheng and Hu, Z. Q.. 2005. "Synthesis and mechanical properties of Cu-based bulk metallic glass composites containing in-situ TiC particles." Scripta Materialia. 52 (7), pp. 669-673. https://doi.org/10.1016/j.scriptamat.2004.10.031Preface to futures in mechanics of structures and materials conference. ACMSM20
Aravinthan, Thiru, Karunasena, Warna (Karu) and Wang, Hao. 2009. "Preface to futures in mechanics of structures and materials conference. ACMSM20." Aravinthan, Thiru, Karunasena, Warna (Karu) and Wang, Hao (ed.) 20th Australasian Conference on the Mechanics of Structures and Materials (ACMSM20). Toowoomba, Australia 02 - 05 Dec 2008 London, United Kingdom.Magnesium thixotropic structure produced by controlled nucleation method
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Wang, Hao. 2007. "In-situ Si/Al composite produced by semisolid metal processing." Materials and Manufacturing Processes. 22 (5-6), pp. 696-699. https://doi.org/10.1080/10426910701384963The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31
Wang, H., Estrin, Y., Fu, H. M., Song, G. L. and Zuberova, Z.. 2007. "The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31." Advanced Engineering Materials. 9 (11), pp. 967-972. https://doi.org/10.1002/adem.200700200Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite
Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498.In situ TiB-reinforced cu-based bulk metallic glass composites
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "In situ TiB-reinforced cu-based bulk metallic glass composites." Scripta Materialia. 54 (11), pp. 1961-1966. https://doi.org/10.1016/j.scriptamat.2006.01.048In-situ Cu-based bulk metallic glass composite
Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2006. "In-situ Cu-based bulk metallic glass composite." International Journal of Modern Physics B. 20 (25-27), pp. 3963-3968. https://doi.org/10.1142/S0217979206040696The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
Yao, X. and Wang, H.. 2006. "Modeling of semisolid structure formation in controlled nucleation method ." International Journal of Modern Physics B. 20 (25-27), pp. 4123-4128. https://doi.org/10.1142/S0217979206040969In-situ Si/Al composite produced by semisolid metal processing
Wang, Hao. 2006. "In-situ Si/Al composite produced by semisolid metal processing ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "Tungsten fibre reinforced Zr-based bulk metallic glass composites ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2007. "Tungsten fibre reinforced Zr-based bulk metallic glass composites." Materials and Manufacturing Processes. 22 (5-6), pp. 687-691. https://doi.org/10.1080/10426910701384922The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ
Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Aravinthan, Thiru. 2010. "The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Sustainable materials research at USQ
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Ning, Z. L., Wang, H., Liu, H. H., Cao, F. Y., Wang, S. T. and Sun, J. F.. 2010. "Effects of Nd on microstructures and properties at the elevated temperature of a Mg-0.3Zn-0.32Zr alloy." Materials and Design. 31 (9), pp. 4438-4444. https://doi.org/10.1016/j.matdes.2010.04.021The role of casting temperature in preparation of bulk metallic glasses
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Li, Qiang, Yu, Baoyi, Zhang, Huawen, Li, Runxia, Wang, Feng, Xie, Shuisheng, Huang, Guojie and Wang, Hao. 2010. "Cellular automaton modeling of semisolid microstructure formation." China Foundry. 7 (2), pp. 143-148.Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites
Kabir, Mohammad Mazedul, Islam, Md Mainul and Wang, Hao. 2010. "Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites." 1st International Conference on Mechanical, Industrial and Energy Engineering (ICMIEE 2010) . Khulna, Bangladesh 23 - 24 Dec 2010 Khulna, Bangladesh.An investigation of spectral response of embedded Fibre Bragg Grating (FBG) sensors in a hollow composite cylindrical beam under pure torsion and combined loading
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Du, Baoxian, Guo, Zhenghong, Song, Pingan, Liu, Hui, Fang, Zhengping and Wu, Yu. 2009. "Flame retardant mechanism of organo-bentonite in polypropylene." Applied Clay Science. 45 (3), pp. 178-184. https://doi.org/10.1016/j.clay.2009.05.003Synthesis of a novel oligomeric intumescent flame retardant and its application in polypropylene
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Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2007. "A practical thermodynamic method to calculate the best glass-forming composition for bulk metallic glasses." International Journal of Nonlinear Sciences and Numerical Simulation. 8 (2), pp. 171-178.Effect of cooling conditions on grain size of AZ91 alloy
Ning, Zhiliang, Cao, P., Wang, Hao, Sun, Jianfei and Liu, Diankun. 2007. "Effect of cooling conditions on grain size of AZ91 alloy." Journal of Materials Science and Technology. 23 (5), pp. 645-649.Effect of pouring temperature on thixotropic microstructure formation of AZ91
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