Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection
Article
Yu, Yueming, Zhang, Yan, Xi, Liangdong, Zhao, Zhinuo, Huo, Siqi, Huang, Guobo, Fang, Zhengping and Song, Pingan. 2022. "Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection." Journal of Cleaner Production. 336, pp. 1-11. https://doi.org/10.1016/j.jclepro.2022.130372
| Article Title | Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection |
|---|---|
| ERA Journal ID | 3639 |
| Article Category | Article |
| Authors | Yu, Yueming (Author), Zhang, Yan (Author), Xi, Liangdong (Author), Zhao, Zhinuo (Author), Huo, Siqi (Author), Huang, Guobo (Author), Fang, Zhengping (Author) and Song, Pingan (Author) |
| Journal Title | Journal of Cleaner Production |
| Journal Citation | 336, pp. 1-11 |
| Article Number | 130372 |
| Number of Pages | 11 |
| Year | 2022 |
| Publisher | Elsevier |
| Place of Publication | Netherlands |
| ISSN | 0959-6526 |
| Digital Object Identifier (DOI) | https://doi.org/10.1016/j.jclepro.2022.130372 |
| Web Address (URL) | https://www.sciencedirect.com/science/article/pii/S095965262200018X |
| Abstract | In this work, we found a very effective method to adjust the polarity of the fillers to promote its good dispersion in matrix by using an organic-solvent-free assembling strategy. With the coating of polyethylenimine-decorated graphene oxide (GO-PEI), the as-prepared biobased core-shell graphene oxide hybrid (BCSGOH) can distribute more homogeneously in the polylactide (PLA) matrix, compared with the bio-derived core-shell flame retardant (CSFR) with higher polarity. The polarity analysis of BCSGOH, CSFR and PLA indicated that the polarity of BCSGOH had a better match with that of PLA, and the interfacial tension (0.8 mN/m) between BCSGOH and PLA was much lower than that (12.0 mN/m) between CSFR and PLA. Consequently, the better flame retardancy, impact toughness and UV-shielding properties of PLA/BCSGOH composites were achieved. 6 wt% of BCSGOH endowed PLA with the best comprehensive properties, such as the UL94 V-0 rating, the limiting oxygen index (LOI) of 30.0%, and notched impact strength of 12.38 kJ/m2. Hence, this work offers a conducive, facile and green strategy to create high-performance fire-safe bioplastics. |
| Keywords | Dispersion; Flame retardancy; Graphene oxide; Polylactide; Toughness |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | NingboTech University, China |
| Taizhou University, China | |
| Centre for Future Materials | |
| Institution of Origin | University of Southern Queensland |
| Funding source | Australian Research Council (ARC) Grant ID DP190102992 |
| Funding source | Australian Research Council (ARC) Grant ID FT190100188 |
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Song, Pingan, Cao, Zhenhu, Cai, Yuanzheng, Zhao, Liping, Fang, Zhengping and Fu, Shenyuan. 2011. "Fabrication of exfoliated graphene-based polypropylene nanocomposites with enhanced mechanical and thermal properties." Polymer. 52 (18), pp. 4001-4010. https://doi.org/10.1016/j.polymer.2011.06.045A novel zinc chelate complex containing both phosphorus and nitrogen for improving the flame retardancy of low density polyethylene
Cao, Zhenhu, Zhang, Yan, Song, Pingan, Cai, Yuanzheng, Guo, Qi, Fang, Zhengping and Peng, Mao. 2011. "A novel zinc chelate complex containing both phosphorus and nitrogen for improving the flame retardancy of low density polyethylene." Journal of Analytical and Applied Pyrolysis. 92 (2), pp. 339-346. https://doi.org/10.1016/j.jaap.2011.07.007Thermal stability and rheological behaviors of high-density polyethylene/fullerene nanocomposites
Zhao, Liping, Song, Ping'An, Cao, Zhenhu, Fang, Zhengping and Guo, Zhenghong. 2012. "Thermal stability and rheological behaviors of high-density polyethylene/fullerene nanocomposites." Journal of Nanomaterials. 2012. https://doi.org/10.1155/2012/340962Effect of lignin incorporation and reactive compatibilization on the morphological, rheological, and mechanical properties of ABS resin
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Yu, Youming, Fu, Shenyuan, Song, Ping'An, Luo, Xiping, Jin, Yongming, Lu, Fengzhu, Wu, Qiang and Ye, Jiewang. 2012. "Functionalized lignin by grafting phosphorus-nitrogen improves the thermal stability and flame retardancy of polypropylene." Polymer Degradation and Stability. 97 (4), pp. 541-546. https://doi.org/10.1016/j.polymdegradstab.2012.01.020Permeability, viscoelasticity, and flammability performances and their relationship to polymer nanocomposites
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Cao, Zhenhu, Song, Pingan, Fang, Zhengping, Xu, Yuanyuan, Zhang, Yan and Guo, Zhenghong. 2012. "Physical wrapping of reduced graphene oxide sheets by polyethylene wax and its modification on the mechanical properties of polyethylene." Journal of Applied Polymer Science. 126 (5), pp. 1546-1555. https://doi.org/10.1002/app.36898Striking multiple synergies created by combining reduced graphene oxides and carbon nanotubes for polymer nanocomposites
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Liu, Lina, Yu, Youming and Song, Ping'An. 2013. "Improved mechanical and thermal properties of polypropylene blends based on diethanolamine-plasticized corn starch via in situ reactive compatibilization." Industrial and Engineering Chemistry Research. 52 (46), pp. 16232-16238. https://doi.org/10.1021/ie4025243Study of the termination of two acrylonitrile radicals and infrared spectrum
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Huang, Guobo, Chen, Suqing, Song, Pingan, Lu, Pingping, Wu, Chenglin and Liang, Huading. 2014. "Combination effects of graphene and layered double hydroxides on intumescent flame-retardant poly(methyl methacrylate) nanocomposites." Applied Clay Science. 88-89, pp. 78-85. https://doi.org/10.1016/j.clay.2013.11.002Combination effect of carbon nanotubes with graphene on intumescent flame-retardant polypropylene nanocomposites
Huang, Guobo, Wang, Shuqu, Song, Ping'An, Wu, Chenglin, Chen, Suqing and Wang, Xu. 2014. "Combination effect of carbon nanotubes with graphene on intumescent flame-retardant polypropylene nanocomposites." Composites Part A: Applied Science and Manufacturing. 59, pp. 18-25. https://doi.org/10.1016/j.compositesa.2013.12.010Evaluating the flammability performance of Portland cement-bonded particleboards with different cement-wood ratios using a cone calorimeter
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Song, Ping'An, Xu, Zhiguang and Guo, Qipeng. 2013. "Bioinspired strategy to reinforce PVA with improved toughness and thermal properties via hydrogen-bond self-assembly." ACS Macro Letters. 2 (12), pp. 1100-1104. https://doi.org/10.1021/mz4005265Synthesis of an intrinsically flame retardant bio-based benzoxazine resin
Yan, Hongquiang, Sun, Chuang, Fang, Zhengping, Liu, Xiaoqing, Zhu, Jin and Wang, Hao. 2016. "Synthesis of an intrinsically flame retardant bio-based benzoxazine resin." Polymer. 97, pp. 418-427. https://doi.org/10.1016/j.polymer.2016.05.053Synthesis of a novel reactive flame retardant containing phosphaphenanthrene and piperidine groups and its application in epoxy resin
Huo, Siqi, Wang, Jun, Yang, Shuang, Zhang, Bin, Chen, Xi, Wu, Qilei and Yang, Lingfeng. 2017. "Synthesis of a novel reactive flame retardant containing phosphaphenanthrene and piperidine groups and its application in epoxy resin." Polymer Degradation and Stability. 146, pp. 250-259. https://doi.org/10.1016/j.polymdegradstab.2017.10.015Enhanced microwave absorption properties of epoxy composites containing graphene decorated with core–shell Fe3O4@polypyrrole nanoparticles
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Huo, Siqi, Wang, Jun, Yang, Shuang, Wang, Junpeng, Zhang, Bin, Zhang, Bo, Chen, Xi and Tang, Yushan. 2016. "Synthesis of a novel phosphorus-nitrogen type flame retardant composed of maleimide, triazine-trione, and phosphaphenanthrene and its flame retardant effect on epoxy resin." Polymer Degradation and Stability. 131, pp. 106-113. https://doi.org/10.1016/j.polymdegradstab.2016.07.013Synergistic flame-retardant effect of expandable graphite and phosphorus-containing compounds for epoxy resin: Strong bonding of different carbon residues
Yang, Shuang, Wang, Jun, Huo, Siqi, Wang, Mei, Wang, Junpeng and Zhang, Bin. 2016. "Synergistic flame-retardant effect of expandable graphite and phosphorus-containing compounds for epoxy resin: Strong bonding of different carbon residues." Polymer Degradation and Stability. 128, pp. 89-98. https://doi.org/10.1016/j.polymdegradstab.2016.03.017Preparation and flame retardancy of DOPO–based epoxy resin containing bismaleimide
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Huo, Siqi, Wang, Jun, Yang, Shuang, Zhang, Bin and Tang, Yushan. 2016. "A phosphorus-containing phenolic derivative and its application in benzoxazine resins: Curing behavior, thermal, and flammability properties." Journal of Applied Polymer Science. 133 (19), pp. 1-7. https://doi.org/10.1002/app.43403Microwave absorption properties of lightweight absorber based on Fe50Ni50-coated poly(acrylonitrile) microspheres and reduced graphene oxide composites
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Wang, Li-li, Zhang, Tao, Yan, Hong-quiang, Peng, Mao, Fang, Zheng-ping, Li, Yan and Wang, Hao. 2014. "Flame-retardant coating by alternate assembly of poly(vinylphosphonic acid) and polyethylenimine for ramie fabrics." Chinese Journal of Polymer Science. 32 (3), pp. 305-314. https://doi.org/10.1007/s10118-014-1408-ySynthesis of a Phosphorus/Nitrogen-Containing Additive with Multifunctional Groups and Its Flame-Retardant Effect in Epoxy Resin
Yang, Shuang, Wang, Jun, Huo, Siqi, Wang, Mei and Cheng, Liufeng. 2015. "Synthesis of a Phosphorus/Nitrogen-Containing Additive with Multifunctional Groups and Its Flame-Retardant Effect in Epoxy Resin." Industrial and Engineering Chemistry Research. 54 (32), pp. 7777-7786. https://doi.org/10.1021/acs.iecr.5b02026The synergistic effect of maleimide and phosphaphenanthrene groups on a reactive flame-retarded epoxy resin system
Yang, Shuang, Wang, Jun, Huo, Siqi, Cheng, Liufeng and Wang, Mei. 2015. "The synergistic effect of maleimide and phosphaphenanthrene groups on a reactive flame-retarded epoxy resin system." Polymer Degradation and Stability. 115, pp. 63-69. https://doi.org/10.1016/j.polymdegradstab.2015.02.016Preparation and flame retardancy of an intumescent flame-retardant epoxy resin system constructed by multiple flame-retardant compositions containing phosphorus and nitrogen heterocycle
Yang, Shuang, Wang, Jun, Huo, Siqi, Cheng, Liufeng and Wang, Mei. 2015. "Preparation and flame retardancy of an intumescent flame-retardant epoxy resin system constructed by multiple flame-retardant compositions containing phosphorus and nitrogen heterocycle." Polymer Degradation and Stability. 119, pp. 251-259. https://doi.org/10.1016/j.polymdegradstab.2015.05.019Preparation and flame retardancy of a compounded epoxy resin system composed of phosphorus/nitrogen-containing active compounds
Yang, Shuang, Wang, Jun, Huo, Siqi, Wang, Mei and Wang, Junpeng. 2015. "Preparation and flame retardancy of a compounded epoxy resin system composed of phosphorus/nitrogen-containing active compounds." Polymer Degradation and Stability. 121, pp. 398-406. https://doi.org/10.1016/j.polymdegradstab.2015.10.006Effect of graphene nanosheets and layered double hydroxides on the flame retardancy and thermal degradation of epoxy resin
Liu, Shan, Yan, Hongqiang, Fang, Zhengping, Guo, Zhenghong and Wang, Hao. 2014. "Effect of graphene nanosheets and layered double hydroxides on the flame retardancy and thermal degradation of epoxy resin." RSC Advances: an international journal to further the chemical sciences. 4 (36), pp. 18652-18659. https://doi.org/10.1039/c4ra01267dThe study of fibre/matrix bond strength in short hemp polypropylene composites from dynamic mechanical analysis
Etaati, Amir, Pather, Selvan, Fang, Zhengping and Wang, Hao. 2014. "The study of fibre/matrix bond strength in short hemp polypropylene composites from dynamic mechanical analysis." Composites Part B: Engineering. 62, pp. 19-28. https://doi.org/10.1016/j.compositesb.2014.02.011Confinement of C60 nanoparticles on the dynamics of polystyrene studied by anelastic spectroscopy and rheometrics
Fang, Zhengping, Shang, Shuying and Wang, Hao. 2013. "Confinement of C60 nanoparticles on the dynamics of polystyrene studied by anelastic spectroscopy and rheometrics." Epaarachchi, Jayantha A. , Lau, Alan Kin-tak and Leng, Jinsong (ed.) 4th International Conference on Smart Materials and Nanotechnology in Engineering (SMN 2013). Gold Coast, Australia 10 - 12 Jul 2013 Bellingham, WA. United States. SPIE. https://doi.org/10.1117/12.2028373Effect of graphene nanosheets on morphology, thermal stability and flame retardancy of epoxy resin
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Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2010. "Effects of corona discharge on the surface structure, morphology and properties of multi-walled carbon nanotubes." Applied Surface Science. 256 (21), pp. 6447-6453. https://doi.org/10.1016/j.apsusc.2010.04.033Biodegradable aliphatic/aromatic copolymers based on terephthalic acid and poly(L-lactic acid): Synthesis, characterization and hydrolytic degradation
Wang, Bing-tao, Zhang, Yan, Song, Pingan, Guo, Zhenghong, Cheng, Jie and Fang, Zhengping. 2010. "Biodegradable aliphatic/aromatic copolymers based on terephthalic acid and poly(L-lactic acid): Synthesis, characterization and hydrolytic degradation." Chinese Journal of Polymer Science. 28 (1), pp. 405-415. https://doi.org/10.1007/s10118-010-9032-yFunctionalization of carbon nanotubes by corona-discharge induced graft polymerization for the reinforcement of epoxy nanocomposites
Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2010. "Functionalization of carbon nanotubes by corona-discharge induced graft polymerization for the reinforcement of epoxy nanocomposites." Plasma Processes and Polymers. 7 (9), pp. 785-793. https://doi.org/10.1002/ppap.201000019Thermal degradation and flammability properties of HDPE/EVA/C60 nanocomposites
Liu, Hui, Song, Pingan, Fang, Zhengping, Shen, Lie and Peng, Mao. 2010. "Thermal degradation and flammability properties of HDPE/EVA/C60 nanocomposites." Thermochimica Acta. 506 (1), pp. 98-101. https://doi.org/10.1016/j.tca.2010.04.029Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites
Fu, Shenyuan, Song, Pingan, Yang, Haitang, Jin, Yongming, Lu, Fengzhu, Ye, Jiewang and Wu, Qiang. 2010. "Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites." Journal of Materials Science. 45 (13), pp. 3520-3528. https://doi.org/10.1007/s10853-010-4394-7Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol
Wang, Bingtao, Zhang, Yan, Song, Pingan, Guo, Zhenghong, Cheng, Jie and Fang, Zhengping. 2010. "Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol." Journal of Applied Polymer Science. 120 (5), pp. 2985-2995. https://doi.org/10.1002/app.33373Flame retardant mechanism of organo-bentonite in polypropylene
Du, Baoxian, Guo, Zhenghong, Song, Pingan, Liu, Hui, Fang, Zhengping and Wu, Yu. 2009. "Flame retardant mechanism of organo-bentonite in polypropylene." Applied Clay Science. 45 (3), pp. 178-184. https://doi.org/10.1016/j.clay.2009.05.003Synthesis of a novel oligomeric intumescent flame retardant and its application in polypropylene
Song, Pingan, Fang, Zhengping, Tong, Lifang and Xu, Zhongbin. 2009. "Synthesis of a novel oligomeric intumescent flame retardant and its application in polypropylene." Polymer Engineering and Science. 48 (7), pp. 1326-1331. https://doi.org/10.1002/pen.21153Fabrication of fullerene (C60) decorated carbon nanotubes and their application in flame-retarding polypropylene
Song, Pingan, Shen, Yu, Du, Baoxian, Guo, Zhenghong and Fang, Zhengping. 2009. "Fabrication of fullerene (C60) decorated carbon nanotubes and their application in flame-retarding polypropylene." Nanoscale. 1 (1), pp. 118-121. https://doi.org/10.1039/B9NR00026GEffects of reactive compatibilization on the morphological, thermal, mechanical and rheological properties of intumescent flame retarded polypropylene
Song, Pingan, Shen, Yu, Du, Baoxian, Peng, Mao, Shen, Lie and Fang, Zhengping. 2009. "Effects of reactive compatibilization on the morphological, thermal, mechanical and rheological properties of intumescent flame retarded polypropylene." ACS Applied Materials and Interfaces. 1 (2), pp. 452-459. https://doi.org/10.1021/am8001204Fabrication of dendrimer-like fullerene (C60) decorated oligomeric intumescent flame retardant for reducing the thermal oxidation and flammability of polypropylene nanocomposites
Song, Pingan, Liu, Hui, Shen, Yu, Du, Baoxian, Fang, Zhengping and Wu, Yu. 2009. "Fabrication of dendrimer-like fullerene (C60) decorated oligomeric intumescent flame retardant for reducing the thermal oxidation and flammability of polypropylene nanocomposites." Journal of Materials Chemistry. 19 (9), pp. 1305-1313. https://doi.org/10.1039/b815610gSurface-initiated graft polymerization on multiwalled carbon nanotubes pretreated by corona discharge at atmospheric pressure
Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2009. "Surface-initiated graft polymerization on multiwalled carbon nanotubes pretreated by corona discharge at atmospheric pressure." Nanoscale. 2 (3), pp. 389-393. https://doi.org/10.1039/B9NR00222GFlame-retardant-wrapped carbon nanotubes for simultaneously improving the flame retardancy and mechanical properties of polypropylene
Song, Ping'an, Xu, Lihua, Guo, Zhenghong, Zhang, Yan and Fang, Zhengping. 2008. "Flame-retardant-wrapped carbon nanotubes for simultaneously improving the flame retardancy and mechanical properties of polypropylene." Journal of Materials Chemistry. 18 (42), pp. 5083-5091. https://doi.org/10.1039/b808309fC60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network
Song, Pingan, Zhu, Yan, Tong, Lifang and Fang, Zhengping. 2008. "C60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network." Nanotechnology. 19 (22). https://doi.org/10.1088/0957-4484/19/22/225707Polypropylene/clay nanocomposites prepared by in situ grafting–melt intercalation with a novel co-intercalating monomer
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