Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection
Article
Yu, Yueming, Zhang, Yan, Xi, Liangdong, Zhao, Zhinuo, Huo, Siqi, Huang, Guobo, Fang, Zhengping and Song, Pingan. 2022. "Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection." Journal of Cleaner Production. 336, pp. 1-11. https://doi.org/10.1016/j.jclepro.2022.130372
| Article Title | Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection |
|---|---|
| ERA Journal ID | 3639 |
| Article Category | Article |
| Authors | Yu, Yueming (Author), Zhang, Yan (Author), Xi, Liangdong (Author), Zhao, Zhinuo (Author), Huo, Siqi (Author), Huang, Guobo (Author), Fang, Zhengping (Author) and Song, Pingan (Author) |
| Journal Title | Journal of Cleaner Production |
| Journal Citation | 336, pp. 1-11 |
| Article Number | 130372 |
| Number of Pages | 11 |
| Year | 2022 |
| Publisher | Elsevier |
| Place of Publication | Netherlands |
| ISSN | 0959-6526 |
| Digital Object Identifier (DOI) | https://doi.org/10.1016/j.jclepro.2022.130372 |
| Web Address (URL) | https://www.sciencedirect.com/science/article/pii/S095965262200018X |
| Abstract | In this work, we found a very effective method to adjust the polarity of the fillers to promote its good dispersion in matrix by using an organic-solvent-free assembling strategy. With the coating of polyethylenimine-decorated graphene oxide (GO-PEI), the as-prepared biobased core-shell graphene oxide hybrid (BCSGOH) can distribute more homogeneously in the polylactide (PLA) matrix, compared with the bio-derived core-shell flame retardant (CSFR) with higher polarity. The polarity analysis of BCSGOH, CSFR and PLA indicated that the polarity of BCSGOH had a better match with that of PLA, and the interfacial tension (0.8 mN/m) between BCSGOH and PLA was much lower than that (12.0 mN/m) between CSFR and PLA. Consequently, the better flame retardancy, impact toughness and UV-shielding properties of PLA/BCSGOH composites were achieved. 6 wt% of BCSGOH endowed PLA with the best comprehensive properties, such as the UL94 V-0 rating, the limiting oxygen index (LOI) of 30.0%, and notched impact strength of 12.38 kJ/m2. Hence, this work offers a conducive, facile and green strategy to create high-performance fire-safe bioplastics. |
| Keywords | Dispersion; Flame retardancy; Graphene oxide; Polylactide; Toughness |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | NingboTech University, China |
| Taizhou University, China | |
| Centre for Future Materials | |
| Institution of Origin | University of Southern Queensland |
| Funding source | Australian Research Council (ARC) Grant ID DP190102992 |
| Funding source | Australian Research Council (ARC) Grant ID FT190100188 |
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Liu, Hui, Song, Pingan, Fang, Zhengping, Shen, Lie and Peng, Mao. 2010. "Thermal degradation and flammability properties of HDPE/EVA/C60 nanocomposites." Thermochimica Acta. 506 (1), pp. 98-101. https://doi.org/10.1016/j.tca.2010.04.029Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites
Fu, Shenyuan, Song, Pingan, Yang, Haitang, Jin, Yongming, Lu, Fengzhu, Ye, Jiewang and Wu, Qiang. 2010. "Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites." Journal of Materials Science. 45 (13), pp. 3520-3528. https://doi.org/10.1007/s10853-010-4394-7Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol
Wang, Bingtao, Zhang, Yan, Song, Pingan, Guo, Zhenghong, Cheng, Jie and Fang, Zhengping. 2010. "Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol." Journal of Applied Polymer Science. 120 (5), pp. 2985-2995. https://doi.org/10.1002/app.33373Flame retardant mechanism of organo-bentonite in polypropylene
Du, Baoxian, Guo, Zhenghong, Song, Pingan, Liu, Hui, Fang, Zhengping and Wu, Yu. 2009. "Flame retardant mechanism of organo-bentonite in polypropylene." Applied Clay Science. 45 (3), pp. 178-184. https://doi.org/10.1016/j.clay.2009.05.003Synthesis of a novel oligomeric intumescent flame retardant and its application in polypropylene
Song, Pingan, Fang, Zhengping, Tong, Lifang and Xu, Zhongbin. 2009. "Synthesis of a novel oligomeric intumescent flame retardant and its application in polypropylene." Polymer Engineering and Science. 48 (7), pp. 1326-1331. https://doi.org/10.1002/pen.21153Fabrication of fullerene (C60) decorated carbon nanotubes and their application in flame-retarding polypropylene
Song, Pingan, Shen, Yu, Du, Baoxian, Guo, Zhenghong and Fang, Zhengping. 2009. "Fabrication of fullerene (C60) decorated carbon nanotubes and their application in flame-retarding polypropylene." Nanoscale. 1 (1), pp. 118-121. https://doi.org/10.1039/B9NR00026GEffects of reactive compatibilization on the morphological, thermal, mechanical and rheological properties of intumescent flame retarded polypropylene
Song, Pingan, Shen, Yu, Du, Baoxian, Peng, Mao, Shen, Lie and Fang, Zhengping. 2009. "Effects of reactive compatibilization on the morphological, thermal, mechanical and rheological properties of intumescent flame retarded polypropylene." ACS Applied Materials and Interfaces. 1 (2), pp. 452-459. https://doi.org/10.1021/am8001204Fabrication of dendrimer-like fullerene (C60) decorated oligomeric intumescent flame retardant for reducing the thermal oxidation and flammability of polypropylene nanocomposites
Song, Pingan, Liu, Hui, Shen, Yu, Du, Baoxian, Fang, Zhengping and Wu, Yu. 2009. "Fabrication of dendrimer-like fullerene (C60) decorated oligomeric intumescent flame retardant for reducing the thermal oxidation and flammability of polypropylene nanocomposites." Journal of Materials Chemistry. 19 (9), pp. 1305-1313. https://doi.org/10.1039/b815610gSurface-initiated graft polymerization on multiwalled carbon nanotubes pretreated by corona discharge at atmospheric pressure
Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2009. "Surface-initiated graft polymerization on multiwalled carbon nanotubes pretreated by corona discharge at atmospheric pressure." Nanoscale. 2 (3), pp. 389-393. https://doi.org/10.1039/B9NR00222GFlame-retardant-wrapped carbon nanotubes for simultaneously improving the flame retardancy and mechanical properties of polypropylene
Song, Ping'an, Xu, Lihua, Guo, Zhenghong, Zhang, Yan and Fang, Zhengping. 2008. "Flame-retardant-wrapped carbon nanotubes for simultaneously improving the flame retardancy and mechanical properties of polypropylene." Journal of Materials Chemistry. 18 (42), pp. 5083-5091. https://doi.org/10.1039/b808309fC60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network
Song, Pingan, Zhu, Yan, Tong, Lifang and Fang, Zhengping. 2008. "C60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network." Nanotechnology. 19 (22). https://doi.org/10.1088/0957-4484/19/22/225707Polypropylene/clay nanocomposites prepared by in situ grafting–melt intercalation with a novel co-intercalating monomer
Song, Pingan, Tong, Lifang and Fang, Zhengping. 2008. "Polypropylene/clay nanocomposites prepared by in situ grafting–melt intercalation with a novel co-intercalating monomer." Journal of Applied Polymer Science. 110 (1), pp. 616-623. https://doi.org/10.1002/app.28689Thermal degradation and flame retardancy of polypropylene/C60 nanocomposites
Fang, Zhengping, Song, Pingan, Tong, Lifang and Guo, Zhenghong. 2008. "Thermal degradation and flame retardancy of polypropylene/C60 nanocomposites." Thermochimica Acta. 473 (1), pp. 106-108. https://doi.org/10.1016/j.tca.2008.04.019Effects of metal chelates on a novel oligomeric intumescent flame retardant system for polypropylene
Song, Pingan, Fang, Zhengping, Tong, Lifang, Jin, Yongming and Lu, Fengzhu. 2008. "Effects of metal chelates on a novel oligomeric intumescent flame retardant system for polypropylene." Journal of Analytical and Applied Pyrolysis. 82 (2), pp. 286-291. https://doi.org/10.1016/j.jaap.2008.04.008Preparation and characterization of hydrophobically modified polyacrylamide hydrogels by grafting glycidyl methacrylate
Song, Pingan, Zhang, Yafeng and Kuang, Jianzheng. 2007. "Preparation and characterization of hydrophobically modified polyacrylamide hydrogels by grafting glycidyl methacrylate." Journal of Materials Science. 42 (8), pp. 2775-2781. https://doi.org/10.1007/s10853-006-1356-1A pH-sensitive Modified Polyacrylamide Hydrogel
Song, Ping An, Zhang, Ya Feng and Kuang, Jian Zheng. 2006. "A pH-sensitive Modified Polyacrylamide Hydrogel." Chinese Chemical Letters. 17 (3), pp. 399-402.This item comprises data from the following sources: Web of Science