Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection
Article
Yu, Yueming, Zhang, Yan, Xi, Liangdong, Zhao, Zhinuo, Huo, Siqi, Huang, Guobo, Fang, Zhengping and Song, Pingan. 2022. "Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection." Journal of Cleaner Production. 336, pp. 1-11. https://doi.org/10.1016/j.jclepro.2022.130372
| Article Title | Interface nanoengineering of a core-shell structured biobased fire retardant for fire-retarding polylactide with enhanced toughness and UV protection |
|---|---|
| ERA Journal ID | 3639 |
| Article Category | Article |
| Authors | Yu, Yueming (Author), Zhang, Yan (Author), Xi, Liangdong (Author), Zhao, Zhinuo (Author), Huo, Siqi (Author), Huang, Guobo (Author), Fang, Zhengping (Author) and Song, Pingan (Author) |
| Journal Title | Journal of Cleaner Production |
| Journal Citation | 336, pp. 1-11 |
| Article Number | 130372 |
| Number of Pages | 11 |
| Year | 2022 |
| Publisher | Elsevier |
| Place of Publication | Netherlands |
| ISSN | 0959-6526 |
| Digital Object Identifier (DOI) | https://doi.org/10.1016/j.jclepro.2022.130372 |
| Web Address (URL) | https://www.sciencedirect.com/science/article/pii/S095965262200018X |
| Abstract | In this work, we found a very effective method to adjust the polarity of the fillers to promote its good dispersion in matrix by using an organic-solvent-free assembling strategy. With the coating of polyethylenimine-decorated graphene oxide (GO-PEI), the as-prepared biobased core-shell graphene oxide hybrid (BCSGOH) can distribute more homogeneously in the polylactide (PLA) matrix, compared with the bio-derived core-shell flame retardant (CSFR) with higher polarity. The polarity analysis of BCSGOH, CSFR and PLA indicated that the polarity of BCSGOH had a better match with that of PLA, and the interfacial tension (0.8 mN/m) between BCSGOH and PLA was much lower than that (12.0 mN/m) between CSFR and PLA. Consequently, the better flame retardancy, impact toughness and UV-shielding properties of PLA/BCSGOH composites were achieved. 6 wt% of BCSGOH endowed PLA with the best comprehensive properties, such as the UL94 V-0 rating, the limiting oxygen index (LOI) of 30.0%, and notched impact strength of 12.38 kJ/m2. Hence, this work offers a conducive, facile and green strategy to create high-performance fire-safe bioplastics. |
| Keywords | Dispersion; Flame retardancy; Graphene oxide; Polylactide; Toughness |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401609. Polymers and plastics | |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | NingboTech University, China |
| Taizhou University, China | |
| Centre for Future Materials | |
| Institution of Origin | University of Southern Queensland |
| Funding source | Australian Research Council (ARC) Grant ID DP190102992 |
| Funding source | Australian Research Council (ARC) Grant ID FT190100188 |
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