Flame retardant and mechanically tough poly(lactic acid) biocomposites via combining ammonia polyphosphate and polyethylene glycol
Article
Sun, Yiqi, Sun, Shuai, Chen, Lei, Liu, Lina, Song, Pingan, Li, Wei, Yu, Youming, Lu, Fengzhu, Qian, Jun and Wang, Hao. 2017. "Flame retardant and mechanically tough poly(lactic acid) biocomposites via combining ammonia polyphosphate and polyethylene glycol." Composites Communications. 6. https://doi.org/10.1016/j.coco.2017.07.005
| Article Title | Flame retardant and mechanically tough poly(lactic acid) biocomposites via combining ammonia polyphosphate and polyethylene glycol |
|---|---|
| ERA Journal ID | 210299 |
| Article Category | Article |
| Authors | Sun, Yiqi (Author), Sun, Shuai (Author), Chen, Lei (Author), Liu, Lina (Author), Song, Pingan (Author), Li, Wei (Author), Yu, Youming (Author), Lu, Fengzhu (Author), Qian, Jun (Author) and Wang, Hao (Author) |
| Journal Title | Composites Communications |
| Journal Citation | 6 |
| Number of Pages | 5 |
| Year | 2017 |
| Publisher | Elsevier |
| Place of Publication | United States |
| ISSN | 2452-2139 |
| Digital Object Identifier (DOI) | https://doi.org/10.1016/j.coco.2017.07.005 |
| Web Address (URL) | https://www.sciencedirect.com/science/article/abs/pii/S2452213917300335 |
| Abstract | Although the flammability of biodegradable poly(lactic acid) (PLA) has been effectively addressed so far, the resultant flame retardant PLA still displays a high brittleness, extremely restricting its wide applications in electrical, automobile and aerospace fields. In this work, we have demonstrated the fabrication of flame retardant and tough PLA composites by combining ammonia polyphosphate (APP) and poly(ethylene glycol) (PEG) with a molecular weight of 20,000 via the melt-blending strategy. The results show that the peak heat release rate of PLA can reduce by 14% in cone tests and a V-0 rating is achieved in vertical burning tests by adding 7 wt% of APP and 14 wt% PEG. Moreover, such PLA composite shows a high strain at break of 280% and impact strength of 14.9 kJ/m2, respectively increasing by thirty-eight-fold and two-fold relative to the PLA bulk. The results strongly indicate that flammability and brittleness of the PLA are strikingly reduced. This work provides an integrated strategy for creating advanced green polymer composites with exceptional flame resistance and toughness. |
| Keywords | flame retardancy; toughness; polylactic acid; ammonia polyphosphate; poly(ethylene glycol) |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 340399. Macromolecular and materials chemistry not elsewhere classified |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | Zhejiang A & F University, China |
| Harbin Institute of Technology, China | |
| Hunan University, China | |
| School of Mechanical and Electrical Engineering | |
| Institution of Origin | University of Southern Queensland |
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Zhuang, Xiao Yu, Chen, Liang, Komarneni, Sridhar, Zhou, Chun Hui, Tong, Dong Shen, Yang, Hui Min, Yu, Wei Hua and Wang, Hao. 2016. "Fly ash-based geopolymer: clean production, properties and applications." Journal of Cleaner Production. 125, pp. 253-267. https://doi.org/10.1016/j.jclepro.2016.03.019Conversion of local industrial wastes into greener cement through geopolymer technology: a case study of high-magnesium nickel slag
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Hua, Fuan, Zhang, Chaoyi, Li, Qiang, Yu, Baoyi, Liu, Weihua, Li, Runxia, Xie, Shuisheng, Huang, Guojie, Cheng, Lei, Fu, Yao and Wang, Hao. 2011. "Numerical simulation of rolling process and microstructure evolution of AM50 Mg alloy during hot rolling process ." Advanced Materials Research. 291-294, pp. 449-454. https://doi.org/10.4028/www.scientific.net/AMR.291-294.449Deformation behaviour of aluminum alloy A356 in semisolid state
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Zhu, Z. W., Zhang, H. F., Wang, H., Ding, B. Z. and Hu, Z. Q.. 2008. "Influence of casting temperature on the thermal stability of Cu- and Zr-based metallic glasses: theoretical analysis and experiments." Journal of Materials Research. 23 (10), pp. 2714-2719. https://doi.org/10.1557/jmr.2008.0335Solidification microstructure modelling using cellular automaton method
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Fu, H. M., Qiu, D., Zhang, M. X., Wang, H., Kelly, P. M. and Taylor, J. A.. 2008. "The development of a new grain refiner for magnesium alloys using the edge-to-edge model." Journal of Alloys and Compounds. 456 (1-2), pp. 390-394. https://doi.org/10.1016/j.jallcom.2007.02.076Cu-based bulk amorphous alloy with larger glass-forming ability and supercooled liquid region
Fu, H. M., Zhang, H. F., Wang, H. and Hu, Z. Q.. 2008. "Cu-based bulk amorphous alloy with larger glass-forming ability and supercooled liquid region." Journal of Alloys and Compounds. 458 (1-2), pp. 390-393. https://doi.org/10.1016/j.jallcom.2007.03.114Study of biodegradation of pure magnesium
Ren, Yibin, Wang, Hao, Huang, Jingjing, Zhang, Bingchun and Yang, Ke. 2007. "Study of biodegradation of pure magnesium." Kim, Young-Ha, Cho, Chong-Su, Kang, Inn-Kyu, Kim, Suk Young and Kwon, Oh Hyeong (ed.) ASBM7: 7th Asian Symposium on Biomedical Materials. Jeju, Korea 20 - 23 Aug 2006 Switzerland. https://doi.org/10.4028/www.scientific.net/KEM.342-343.601The use of simulated games in an undergraduate course manufacturing processes
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Yao, Xiangdong, Wang, Hao, He, B. and Zhou, X.. 2005. "Modeling of columnar-to-equiaxed transition in solidified Al-Si alloys." Zhong, Z., Saka, H., Kim, T. H., Holm, E. A., Han, Y. and Xie, X. (ed.) 5th Pacific Rim International Conference on Advanced Materials and Processing (PRICM 5). Beijing, China 02 - 05 Nov 2004 Zurich, Switzerland. Scientific.Net. https://doi.org/10.4028/www.scientific.net/MSF.475-479.3141Formation and mechanical properties of Mg65Cu25Er10 and Mg65Cu15Ag10Er10 bulk amorphous alloys
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Fu, H. M., Zhang, H. F., Wang, Hao, Zhang, Qingsheng and Hu, Z. Q.. 2005. "Synthesis and mechanical properties of Cu-based bulk metallic glass composites containing in-situ TiC particles." Scripta Materialia. 52 (7), pp. 669-673. https://doi.org/10.1016/j.scriptamat.2004.10.031Preface to futures in mechanics of structures and materials conference. ACMSM20
Aravinthan, Thiru, Karunasena, Warna (Karu) and Wang, Hao. 2009. "Preface to futures in mechanics of structures and materials conference. ACMSM20." Aravinthan, Thiru, Karunasena, Warna (Karu) and Wang, Hao (ed.) 20th Australasian Conference on the Mechanics of Structures and Materials (ACMSM20). Toowoomba, Australia 02 - 05 Dec 2008 London, United Kingdom.Magnesium thixotropic structure produced by controlled nucleation method
Wang, Hao and Ning, Zhiliang. 2007. "Magnesium thixotropic structure produced by controlled nucleation method ." Tezhong Zhuzao Ji Youse Hejin (Special Casting and Nonferrous Alloys).In-situ Si/Al composite produced by semisolid metal processing
Wang, Hao. 2007. "In-situ Si/Al composite produced by semisolid metal processing." Materials and Manufacturing Processes. 22 (5-6), pp. 696-699. https://doi.org/10.1080/10426910701384963The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31
Wang, H., Estrin, Y., Fu, H. M., Song, G. L. and Zuberova, Z.. 2007. "The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31." Advanced Engineering Materials. 9 (11), pp. 967-972. https://doi.org/10.1002/adem.200700200Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite
Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498.In situ TiB-reinforced cu-based bulk metallic glass composites
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Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2006. "In-situ Cu-based bulk metallic glass composite." International Journal of Modern Physics B. 20 (25-27), pp. 3963-3968. https://doi.org/10.1142/S0217979206040696The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
Yao, X. and Wang, H.. 2006. "Modeling of semisolid structure formation in controlled nucleation method ." International Journal of Modern Physics B. 20 (25-27), pp. 4123-4128. https://doi.org/10.1142/S0217979206040969In-situ Si/Al composite produced by semisolid metal processing
Wang, Hao. 2006. "In-situ Si/Al composite produced by semisolid metal processing ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "Tungsten fibre reinforced Zr-based bulk metallic glass composites ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2007. "Tungsten fibre reinforced Zr-based bulk metallic glass composites." Materials and Manufacturing Processes. 22 (5-6), pp. 687-691. https://doi.org/10.1080/10426910701384922The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ
Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Aravinthan, Thiru. 2010. "The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Sustainable materials research at USQ
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Zhu, Zhengwang, Zhang, Haifeng, Wang, Hao, Ding, Bingzhe, Hu, Zhuang-Qi and Huang, Han. 2009. "Influence of casting temperature on microstructures and mechanical properties of Cu50Zr45.5Ti2.5Y2 metallic glass prepared using copper mold casting [+ Erratum]." Journal of Materials Research. 24 (10), pp. 3108-3115. https://doi.org/10.1557/jmr.2009.0373Deformation behavior of semisolid A356 alloy prepared by low temperature pouring
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Ning, Z. L., Wang, H., Liu, H. H., Cao, F. Y., Wang, S. T. and Sun, J. F.. 2010. "Effects of Nd on microstructures and properties at the elevated temperature of a Mg-0.3Zn-0.32Zr alloy." Materials and Design. 31 (9), pp. 4438-4444. https://doi.org/10.1016/j.matdes.2010.04.021The role of casting temperature in preparation of bulk metallic glasses
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Li, Qiang, Yu, Baoyi, Zhang, Huawen, Li, Runxia, Wang, Feng, Xie, Shuisheng, Huang, Guojie and Wang, Hao. 2010. "Cellular automaton modeling of semisolid microstructure formation." China Foundry. 7 (2), pp. 143-148.Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites
Kabir, Mohammad Mazedul, Islam, Md Mainul and Wang, Hao. 2010. "Mechanical and thermal properties of untreated and chemically treated jute fibre reinforced composites." 1st International Conference on Mechanical, Industrial and Energy Engineering (ICMIEE 2010) . Khulna, Bangladesh 23 - 24 Dec 2010 Khulna, Bangladesh.An investigation of spectral response of embedded Fibre Bragg Grating (FBG) sensors in a hollow composite cylindrical beam under pure torsion and combined loading
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Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Canning, John. 2010. "Effects of the self distortions of embedded FBG sensors on spectral response due to torsional and combined loads." 3rd Asia-Pacific Workshop on Structural Health Monitoring (APWSHM 2010). Tokyo, Japan 30 Nov - 02 Dec 2010 Tokyo, Japan.Natural fibre composites with epoxidized vegetable oil (EVO) resins: a review
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Ren, Yibin, Huang, Jingjing, Yang, Ke, Zhang, Bingchun, Yao, Zhiming and Wang, Hao. 2005. "Study of bio-corrosion of pure magnesium." Jinshu Xuebao. 41 (11), pp. 1228-1232.Present status and future trends in production of semisolid materials
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Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2010. "Functionalization of carbon nanotubes by corona-discharge induced graft polymerization for the reinforcement of epoxy nanocomposites." Plasma Processes and Polymers. 7 (9), pp. 785-793. https://doi.org/10.1002/ppap.201000019Thermal degradation and flammability properties of HDPE/EVA/C60 nanocomposites
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Fu, Shenyuan, Song, Pingan, Yang, Haitang, Jin, Yongming, Lu, Fengzhu, Ye, Jiewang and Wu, Qiang. 2010. "Effects of carbon nanotubes and its functionalization on the thermal and flammability properties of polypropylene wood flour composites." Journal of Materials Science. 45 (13), pp. 3520-3528. https://doi.org/10.1007/s10853-010-4394-7Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol
Wang, Bingtao, Zhang, Yan, Song, Pingan, Guo, Zhenghong, Cheng, Jie and Fang, Zhengping. 2010. "Synthesis, characterization, and properties of degradable poly(l-lactic acid)/poly(butylene terephthalate) copolyesters containing 1,4-cyclohexanedimethanol." Journal of Applied Polymer Science. 120 (5), pp. 2985-2995. https://doi.org/10.1002/app.33373Use of wireless tablet PCs as an effective learning and teaching enhancement tool
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Du, Baoxian, Guo, Zhenghong, Song, Pingan, Liu, Hui, Fang, Zhengping and Wu, Yu. 2009. "Flame retardant mechanism of organo-bentonite in polypropylene." Applied Clay Science. 45 (3), pp. 178-184. https://doi.org/10.1016/j.clay.2009.05.003Synthesis of a novel oligomeric intumescent flame retardant and its application in polypropylene
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Xu, Lihua, Fang, Zhengping, Song, Pingan and Peng, Mao. 2009. "Surface-initiated graft polymerization on multiwalled carbon nanotubes pretreated by corona discharge at atmospheric pressure." Nanoscale. 2 (3), pp. 389-393. https://doi.org/10.1039/B9NR00222GDevelopment of bulk metallic glass composites
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