Bioinspired, Highly Adhesive, Nanostructured Polymeric Coatings for Superhydrophobic Fire-Extinguishing Thermal Insulation Foam
Article
Ma, Zhewen, Liu, Xiaochen, Xu, Xiaodong, Liu, Lei, Yu, Bin, Maluk, Cristian, Huang, Guobo, Wang, Hao and Song, Pingan. 2021. "Bioinspired, Highly Adhesive, Nanostructured Polymeric Coatings for Superhydrophobic Fire-Extinguishing Thermal Insulation Foam." ACS Nano. 15 (7), pp. 11667-11680. https://doi.org/10.1021/acsnano.1c02254
| Article Title | Bioinspired, Highly Adhesive, Nanostructured Polymeric Coatings for Superhydrophobic Fire-Extinguishing Thermal Insulation Foam |
|---|---|
| ERA Journal ID | 35029 |
| Article Category | Article |
| Authors | Ma, Zhewen (Author), Liu, Xiaochen (Author), Xu, Xiaodong (Author), Liu, Lei (Author), Yu, Bin (Author), Maluk, Cristian (Author), Huang, Guobo (Author), Wang, Hao (Author) and Song, Pingan (Author) |
| Journal Title | ACS Nano |
| Journal Citation | 15 (7), pp. 11667-11680 |
| Number of Pages | 14 |
| Year | 2021 |
| Publisher | American Chemical Society |
| Place of Publication | United States |
| ISSN | 1936-0851 |
| 1936-086X | |
| Digital Object Identifier (DOI) | https://doi.org/10.1021/acsnano.1c02254 |
| Web Address (URL) | https://pubs.acs.org/doi/10.1021/acsnano.1c02254 |
| Abstract | Lightweight polymeric foam is highly attractive as thermal insulation materials for energy-saving buildings but is plagued by its inherent flammability. Fire-retardant coatings are suggested as an effective means to solve this problem. However, most of the existing fire-retardant coatings suffer from poor interfacial adhesion to polymeric foam during use. In nature, snails and tree frogs exhibit strong adhesion to a variety of surfaces by interfacial hydrogen-bonding and mechanical interlocking, respectively. Inspired by their adhesion mechanisms, we herein rationally design fire-retardant polymeric coatings with phase-separated micro/nanostructures via a facile radical copolymerization of hydroxyethyl acrylate (HEA) and sodium vinylsulfonate (VS). The resultant waterborne poly(VS-co-HEA) copolymers exhibit strong interfacial adhesion to rigid polyurethane (PU) foam and other substrates, better than most of the current adhesives because of the combination of interfacial hydrogen-bonding and mechanical interlocking. Besides a superhydrophobic feature, the poly(VS-co-HEA)-coated PU foam can self-extinguish a flame, exhibiting a desired V-0 rating during vertical burning and low heat and smoke release due to its high charring capability, which is superior to its previous counterparts. Moreover, the foam thermal insulation is well-preserved and agrees well with theoretical calculations. This work offers a facile biomimetic strategy for creating advanced adhesive fire-retardant polymeric coatings for many flammable substrates. |
| Keywords | Energy-saving buildings; Fire retardant coating; Hydroxyethyl acrylate; Interfacial adhesions; Mechanical interlocking; Radical copolymerization; Theoretical calculations; Thermal insulation materials |
| Contains Sensitive Content | Does not contain sensitive content |
| ANZSRC Field of Research 2020 | 401605. Functional materials |
| 401602. Composite and hybrid materials | |
| Public Notes | Files associated with this item cannot be displayed due to copyright restrictions. |
| Byline Affiliations | Zhejiang A & F University, China |
| Henan Normal University, China | |
| University of Science and Technology of China, Hefei, China | |
| University of Queensland | |
| Taizhou University, China | |
| Centre for Future Materials | |
| Institution of Origin | University of Southern Queensland |
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Ren, Yibin, Wang, Hao, Huang, Jingjing, Zhang, Bingchun and Yang, Ke. 2007. "Study of biodegradation of pure magnesium." Kim, Young-Ha, Cho, Chong-Su, Kang, Inn-Kyu, Kim, Suk Young and Kwon, Oh Hyeong (ed.) ASBM7: 7th Asian Symposium on Biomedical Materials. Jeju, Korea 20 - 23 Aug 2006 Switzerland. https://doi.org/10.4028/www.scientific.net/KEM.342-343.601The use of simulated games in an undergraduate course manufacturing processes
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Fu, H. M., Zhang, H. F., Wang, Hao, Zhang, Qingsheng and Hu, Z. Q.. 2005. "Synthesis and mechanical properties of Cu-based bulk metallic glass composites containing in-situ TiC particles." Scripta Materialia. 52 (7), pp. 669-673. https://doi.org/10.1016/j.scriptamat.2004.10.031Preface to futures in mechanics of structures and materials conference. ACMSM20
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Wang, H., Estrin, Y., Fu, H. M., Song, G. L. and Zuberova, Z.. 2007. "The effect of pre-processing and grain structure on the bio-corrosion and fatigue resistance of magnesium alloy AZ31." Advanced Engineering Materials. 9 (11), pp. 967-972. https://doi.org/10.1002/adem.200700200Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite
Yao, X. D., Wu, C. Z., Wang, Hao, Cheng, H. M. and Lu, G. Q.. 2006. "Effects of carbon nanotubes and metal catalysts on hydrogen storage in magnesium nanocomposite." Journal of Nanoscience and Nanotechnology. 6 (2), pp. 494-498.In situ TiB-reinforced cu-based bulk metallic glass composites
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "In situ TiB-reinforced cu-based bulk metallic glass composites." Scripta Materialia. 54 (11), pp. 1961-1966. https://doi.org/10.1016/j.scriptamat.2006.01.048In-situ Cu-based bulk metallic glass composite
Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2006. "In-situ Cu-based bulk metallic glass composite." International Journal of Modern Physics B. 20 (25-27), pp. 3963-3968. https://doi.org/10.1142/S0217979206040696The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy
Fu, H. M., Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "The effect of Gd addition on the glass-forming ability of Cu-Zr-Al alloy." Scripta Materialia. 55 (2), pp. 147-150. https://doi.org/10.1016/j.scriptamat.2006.03.052Modeling of semisolid structure formation in controlled nucleation method
Yao, X. and Wang, H.. 2006. "Modeling of semisolid structure formation in controlled nucleation method ." International Journal of Modern Physics B. 20 (25-27), pp. 4123-4128. https://doi.org/10.1142/S0217979206040969In-situ Si/Al composite produced by semisolid metal processing
Wang, Hao. 2006. "In-situ Si/Al composite produced by semisolid metal processing ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2006. "Tungsten fibre reinforced Zr-based bulk metallic glass composites ." Bandyopadhyay, Sri, Zeng, Q., Berndt, Christopher C., Rizkalla, S., Gowripalan, N. and Matison, Janison (ed.) ACUN-5 International Composites Conference. Sydney, Australia 11 - 14 Jul 2006 Sydney, Australia.Tungsten fibre reinforced Zr-based bulk metallic glass composites
Wang, Hao, Zhang, H. F. and Hu, Z. Q.. 2007. "Tungsten fibre reinforced Zr-based bulk metallic glass composites." Materials and Manufacturing Processes. 22 (5-6), pp. 687-691. https://doi.org/10.1080/10426910701384922The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ
Kahandawa, Gayan C., Epaarachchi, Jayantha A., Wang, Hao and Aravinthan, Thiru. 2010. "The developments of structural health/integrity monitoring systems using FBG sensors at CEEFC of USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia.Sustainable materials research at USQ
Wang, Hao. 2010. "Sustainable materials research at USQ." Goh, Steven C. and Wang, Hao (ed.) 2010 Southern Region Engineering Conference (SREC 2010). Toowoomba, Australia 11 - 12 Nov 2010 Toowoomba, Australia .Influence of casting temperature on microstructures and mechanical properties of Cu50Zr45.5Ti2.5Y2 metallic glass prepared using copper mold casting [+ Erratum]
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Ning, Z. L., Wang, H., Liu, H. H., Cao, F. Y., Wang, S. T. and Sun, J. F.. 2010. "Effects of Nd on microstructures and properties at the elevated temperature of a Mg-0.3Zn-0.32Zr alloy." Materials and Design. 31 (9), pp. 4438-4444. https://doi.org/10.1016/j.matdes.2010.04.021The role of casting temperature in preparation of bulk metallic glasses
Wang, Hao. 2010. "The role of casting temperature in preparation of bulk metallic glasses ." Chandra, T., Wanderka, N., Reimers, W. and Ionescu, M. (ed.) 6th International Conference on Processing and Manufacturing of Advanced Materials (THERMEC 2009): Processing, Fabrication, Properties, Applications. Berlin, Germany 25 - 29 Aug 2009 Switzerland. https://doi.org/10.4028/www.scientific.net/MSF.638-642.1671Characteristics of a silk fibre reinforced biodegradable plastic
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Wang, Hao. 2005. "Semisolid structure formation and semisolid casting." Journal of Materials Science and Technology. 21 (1 (Supplement)), pp. 65-71.Multifarious fracture features of CuZrAlGd(Ag) bulk metallic glasses
Fu, H. M., Zhang, H. F., Wang, Hao and Hu, Z. Q.. 2007. "Multifarious fracture features of CuZrAlGd(Ag) bulk metallic glasses." Advanced Materials Research. 29-30, pp. 47-50.A practical thermodynamic method to calculate the best glass-forming composition for bulk metallic glasses
Wang, Hao, Fu, H. M., Zhang, H. F. and Hu, Z. Q.. 2007. "A practical thermodynamic method to calculate the best glass-forming composition for bulk metallic glasses." International Journal of Nonlinear Sciences and Numerical Simulation. 8 (2), pp. 171-178.Effect of cooling conditions on grain size of AZ91 alloy
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Ning, Zhiliang, Wu, Peilian, Wang, Hao, Cao, Fuyang and Sun, Jianfei. 2007. "Effect of pouring temperature on thixotropic microstructure formation of AZ91." Rare Metals. 26 (S1), pp. 180-184.Bulk metallic glass composites
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Song, Ping'an, Xu, Lihua, Guo, Zhenghong, Zhang, Yan and Fang, Zhengping. 2008. "Flame-retardant-wrapped carbon nanotubes for simultaneously improving the flame retardancy and mechanical properties of polypropylene." Journal of Materials Chemistry. 18 (42), pp. 5083-5091. https://doi.org/10.1039/b808309fC60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network
Song, Pingan, Zhu, Yan, Tong, Lifang and Fang, Zhengping. 2008. "C60 reduces the flammability of polypropylene nanocomposites by in situ forming gelled-ball network." Nanotechnology. 19 (22). https://doi.org/10.1088/0957-4484/19/22/225707Polypropylene/clay nanocomposites prepared by in situ grafting–melt intercalation with a novel co-intercalating monomer
Song, Pingan, Tong, Lifang and Fang, Zhengping. 2008. "Polypropylene/clay nanocomposites prepared by in situ grafting–melt intercalation with a novel co-intercalating monomer." Journal of Applied Polymer Science. 110 (1), pp. 616-623. https://doi.org/10.1002/app.28689Thermal degradation and flame retardancy of polypropylene/C60 nanocomposites
Fang, Zhengping, Song, Pingan, Tong, Lifang and Guo, Zhenghong. 2008. "Thermal degradation and flame retardancy of polypropylene/C60 nanocomposites." Thermochimica Acta. 473 (1), pp. 106-108. https://doi.org/10.1016/j.tca.2008.04.019Effects of metal chelates on a novel oligomeric intumescent flame retardant system for polypropylene
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