Phase transformation and negative thermal expansion in TaVO5

Article

Wang, Xiaowei, Huang, Qingzhen, Deng, Jinxia, Yu, Ranbo, Chen, Jun and Xing, Xianran. 2011. "Phase transformation and negative thermal expansion in TaVO5." Inorganic Chemistry: including bioinorganic chemistry. 50 (6), pp. 2685-2690. https://doi.org/10.1021/ic200003n
Article Title

Phase transformation and negative thermal expansion in TaVO5

ERA Journal ID1525
Article CategoryArticle
AuthorsWang, Xiaowei (Author), Huang, Qingzhen (Author), Deng, Jinxia (Author), Yu, Ranbo (Author), Chen, Jun (Author) and Xing, Xianran (Author)
Journal TitleInorganic Chemistry: including bioinorganic chemistry
Journal Citation50 (6), pp. 2685-2690
Number of Pages6
Year2011
Place of PublicationUnited States
ISSN0020-1669
1520-510X
Digital Object Identifier (DOI)https://doi.org/10.1021/ic200003n
Web Address (URL)http://pubs.acs.org/doi/abs/10.1021/ic200003n
Abstract

Two phase transformations of TaVO5 were observed by DSC and/or dilatometry measurements in the studied temperature range. X-ray diffraction and neutron powder diffraction structure refinements indicated a phase transformation at-14 °C from a monoclinic symmetry with space group P2 1/c to an orthorhombic symmetry with space group Pnma above this temperature. The rigid TaO6 octahedron in orthorhombic phase becomes nonregular at-14 °C, which results in the transition from Pnma to P2 1/c. TaVO5 was found to be a negative thermal expansion material above room temperature. The calculated volumetric thermal expansion coefficients (TECs) are-8.92 × 10-6 °C-1 in the range of 20-600 °C, and-2.19 × 10-5 °C-1 above 600 °C, respectively. The negative thermal expansion behavior is accounted for by the tilt of the TaO6 and VO4 polyhedra, where the shrinkage of the VO4 tetrahedra result in the increase of Ta-O-V angles on heating, while the angle of Ta-O1-Ta maintains at 180° in the framework.

ANZSRC Field of Research 2020340201. Bioinorganic chemistry
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Byline AffiliationsUniversity of Science and Technology Beijing, China
National Institute of Standards and Technology, United States
Institution of OriginUniversity of Southern Queensland
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Wang, Feng, Wang, Jiangyan, Ren, Hao, Tang, Hongjie, Yu, Ranbo and Wang, Dan. 2016. "Multi-shelled LiMn2O4 hollow microspheres as superior cathode materials for lithium-ion batteries." Inorganic Chemistry Frontiers. 3 (3), pp. 365-369. https://doi.org/10.1039/c5qi00213c
Facile solvothermal synthesis of gear-shaped submicrostructured Y2O3:Eu 3+ phosphor
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The role of spontaneous polarization in the negative thermal expansion of tetragonal PbTiO3-based compounds
Chen, Jun, Nittala, Krishna, Forrester, Jennifer S., Jones, Jacob L., Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2011. "The role of spontaneous polarization in the negative thermal expansion of tetragonal PbTiO3-based compounds." Journal of the American Chemical Society. 133 (29), pp. 11114-11117. https://doi.org/10.1021/ja2046292
Facile molten salt synthesis of ordered perovskite Ba(Sr 1/3Nb 2/3)O3 powders
Deng, Jinxia, Li, Lihong, Chen, Jun, Yu, Ranbo and Xing, Xianran. 2012. "Facile molten salt synthesis of ordered perovskite Ba(Sr 1/3Nb 2/3)O3 powders." Inorganic Chemistry Communications. 21, pp. 92-95. https://doi.org/10.1016/j.inoche.2012.04.021
Morphology-tailored synthesis of flower-like Y 2O 3:Eu3+ microspheres
Yan, Xuecheng, Yu, Ranbo, Xu, Yali, Li, Li, Xu, Pengfei, Wang, Dan, Deng, Jinxia, Chen, Jun and Xing, Xianran. 2012. "Morphology-tailored synthesis of flower-like Y 2O 3:Eu3+ microspheres." Materials Research Bulletin. 47 (9), pp. 2135-2139. https://doi.org/10.1016/j.materresbull.2012.06.013
Rapid molten salt synthesis of isotropic negative thermal expansion ScF3
Hu, Lei, Chen, Jun, Fan, Longlong, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2014. "Rapid molten salt synthesis of isotropic negative thermal expansion ScF3." Journal of the American Ceramic Society. 97 (4), pp. 1009-1011. https://doi.org/10.1111/jace.12855
Large-scale synthesis of isotropic single-crystalline ScF3 cubes by hydrothermal method
Hu, Lei, Chen, Jun, Pan, Zhao, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2014. "Large-scale synthesis of isotropic single-crystalline ScF3 cubes by hydrothermal method." Journal of the American Ceramic Society. 97 (5), pp. 1386-1388. https://doi.org/10.1111/jace.12932
Zero thermal expansion and ferromagnetism in cubic sc1-xMxF3 (M = Ga, Fe) over a wide temperature range
Hu, Lei, Chen, Jun, Fan, Longlong, Ren, Yang, Rong, Yangchun, Pan, Zhao, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2014. "Zero thermal expansion and ferromagnetism in cubic sc1-xMxF3 (M = Ga, Fe) over a wide temperature range." Journal of the American Chemical Society. 136 (39), pp. 13566-13569. https://doi.org/10.1021/ja5077487
Controlled synthesis and properties of porous Cu/CeO2 microspheres
Yao, Xiang, Yang, Xiaodan, Yu, Ranbo, Xu, Pengfei, Chen, Jun and Xing, Xianran. 2015. "Controlled synthesis and properties of porous Cu/CeO2 microspheres." Materials Research Bulletin. 61, pp. 22-25. https://doi.org/10.1016/j.materresbull.2014.09.083
Controllable assembly of CeO2 micro/nanospheres with adjustable size and their application in Cr(VI) adsorption
Sun, Jiajia, Wang, Chengrui, Zeng, Li, Xu, Pengfei, Yang, Xiaodan, Chen, Jun, Xing, Xianran, Jin, Quan and Yu, Ranbo. 2016. "Controllable assembly of CeO2 micro/nanospheres with adjustable size and their application in Cr(VI) adsorption." Materials Research Bulletin. 75, pp. 110-114. https://doi.org/10.1016/j.materresbull.2015.11.035
N,N-dimethylformamide-induced synthesis and photoluminescence of CePO4 and Ce0.95PO4:Tb0.05 with sphere-like nanostructures
Bao, Jinrong, Zhu, Xiaowei, Liu, Ying, Li, Wenxian and Yu, Ranbo. 2014. "N,N-dimethylformamide-induced synthesis and photoluminescence of CePO4 and Ce0.95PO4:Tb0.05 with sphere-like nanostructures." Materials Letters. 124, pp. 97-100. https://doi.org/10.1016/j.matlet.2014.03.014
Microstructure construction and composition modification of CeO2 macrospheres with superior performance
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Bismuth oxychloride hollow microspheres with high visible light photocatalytic activity
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A novel and highly efficient photocatalyst based on P 25- graphdiyne nanocomposite
Wang, Shuo, Yi, Luoxin, Halpert, Jonathan E., Lai, Xiaoyong, Liu, Yuanyuan, Cao, Hongbin, Wang, Dan, Yu, Ranbo and Li, Yuliang. 2012. "A novel and highly efficient photocatalyst based on P 25- graphdiyne nanocomposite." Small. 8 (2), pp. 265-271. https://doi.org/10.1002/smll.201101686
Study on the controllable scale-up growth of vertically-aligned carbon nanotube arrays
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Embeddable and locatable spinning
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Finite element analysis of eroding type surface thermocouple with application to engine heat flux measurement
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