Bismuth oxychloride hollow microspheres with high visible light photocatalytic activity

Article

Cui, Pengzhen, Wang, Jiali, Wang, Zumin, Chen, Jun, Xing, Xianran, Wang, Lianzhou and Yu, Ranbo. 2016. "Bismuth oxychloride hollow microspheres with high visible light photocatalytic activity." Nano Research. 9 (3), pp. 593-601. https://doi.org/10.1007/s12274-015-0939-z
Article Title

Bismuth oxychloride hollow microspheres with high visible light photocatalytic activity

ERA Journal ID123989
Article CategoryArticle
AuthorsCui, Pengzhen (Author), Wang, Jiali (Author), Wang, Zumin (Author), Chen, Jun (Author), Xing, Xianran (Author), Wang, Lianzhou (Author) and Yu, Ranbo (Author)
Journal TitleNano Research
Journal Citation9 (3), pp. 593-601
Number of Pages9
Year2016
PublisherSpringer
Place of PublicationChina
ISSN1998-0000
1998-0124
Digital Object Identifier (DOI)https://doi.org/10.1007/s12274-015-0939-z
Web Address (URL)https://link.springer.com/article/10.1007%2Fs12274-015-0939-z
Abstract

Hollow microspheres of two bismuth oxychlorides, BiOCl and Bi24O31Cl10, were successfully synthesized using carbonaceous microsphere sacrificial templates. The phase evolution from BiOCl to Bi24O31Cl10 was easily realized by heating the former at 600 °C. With a uniform diameter of about 200 nm, an average shell thickness of 40 nm, and basic nanosheets of <20 nm, the hollow microspheres of both BiOCl and Bi24O31Cl10 showed high visible light photocatalytic activity towards the degradation of Rhodamine B (RhB). Besides the effective photosensitization process and efficient photointroduced carrier separation, the high photocatalytic activity was believed to result from their hollow-structure-dependent large visible light absorption. Moreover, as a chlorine-deficient analogue, the Bi24O31Cl10 hollow spheres possessed a narrower band gap, more dispersive band structure, and higher photocarrier conversion efficiency, which further helped them to exhibit better photocatalytic activity. [Figure not available: see fulltext.]

Keywordsbismuth oxychloride; hollow spheres; nanosturctures; visible light photocatalysis; Bismuth oxychloride; High photocatalytic activities; Hollow sphere; nanosturctures; Photocatalytic activities; Visible light absorption; Visible light photocatalytic activity; Visible-light photocatalysis;
ANZSRC Field of Research 2020401899. Nanotechnology not elsewhere classified
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Byline AffiliationsUniversity of Science and Technology Beijing, China
University of Queensland
Institution of OriginUniversity of Southern Queensland
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A new graphdiyne nanosheet/Pt nanoparticle-based counter electrode material with enhanced catalytic activity for dye-sensitized solar cells
Ren, Hao, Shao, Hui, Zhang, Lijuan, Guo, Dong, Jin, Quan, Yu, Ranbo, Wang, Lei, Li, Yuliang, Wang, Yun, Zhao, Huijun and Wang, Dan. 2015. "A new graphdiyne nanosheet/Pt nanoparticle-based counter electrode material with enhanced catalytic activity for dye-sensitized solar cells." Advanced Energy Materials. 5 (12). https://doi.org/10.1002/aenm.201500296
Controllable synthesis of mesostructures from TiO2 hollow to porous nanospheres with superior rate performance for lithium ion batteries
Ren, Hao, Sun, Jiajia, Yu, Ranbo, Yang, Mei, Gu, Lin, Liu, Porun, Zhao, Huijun, Kisailus, David and Wang, Dan. 2015. "Controllable synthesis of mesostructures from TiO2 hollow to porous nanospheres with superior rate performance for lithium ion batteries." Chemical Science. 7 (1), pp. 793-798. https://doi.org/10.1039/c5sc03203b
Multiple Au cores in CeO2 hollow spheres for the superior catalytic reduction of p-nitrophenol
Zhao, Kun, Qi, Jian, Zhao, Shenlong, Tang, Hongjie, Yin, Huajie, Zong, Lingbo, Chang, Lin, Gao, Yan, Yu, Ranbo and Tang, Zhiyong. 2015. "Multiple Au cores in CeO2 hollow spheres for the superior catalytic reduction of p-nitrophenol." Chinese Journal of Catalysis. 36 (3), pp. 261-267. https://doi.org/10.1016/S1872-2067(14)60273-4
Y203:Yb3+/Er3+ hollow spheres with controlled inner structures and enhanced upconverted photoluminescence
Zong, Lingbo, Xu, Pengfei, Ding, Yunji, Zhao, Kun, Wang, Zumin, Yan, Xuecheng, Yu, Ranbo, Chen, Jun and Xing, Xianran. 2015. "Y203:Yb3+/Er3+ hollow spheres with controlled inner structures and enhanced upconverted photoluminescence." Small. 11 (23), pp. 2768-2773. https://doi.org/10.1002/smll.201402320
Controlled synthesis of tetragonal terbium orthophosphate nanostructures through a solvothermal route
Yu, Ranbo, Bao, Jinrong, Yang, Xiaodan, Zhang, Jiayun, Deng, Jinxia, Chen, Jun and Xing, Xianran. 2011. "Controlled synthesis of tetragonal terbium orthophosphate nanostructures through a solvothermal route." Research on Chemical Intermediates. 37 (2-5), pp. 145-151. https://doi.org/10.1007/s11164-011-0261-7
Hierarchical hydroxyapatite microspheres composed of nanorods and their competitive sorption behavior for heavy metal ions
Zhu, Ronghai, Lai, Xiaoyong, Halpert, Jonathan E., Yu, Ranbo and Wang, Dan. 2012. "Hierarchical hydroxyapatite microspheres composed of nanorods and their competitive sorption behavior for heavy metal ions." European Journal of Inorganic Chemistry. https://doi.org/10.1002/ejic.201101038
Water-soluble monodispersed lanthanide oxide submicrospheres: PVP-assisted hydrothermal synthesis, size-control and luminescence properties
Cui, Ying, Lai, Xiaoyong, Li, Li, Hu, Zhudong, Wang, Shuo, Halpert, Jonathan E., Yu, Ranbo and Wang, Dan. 2012. "Water-soluble monodispersed lanthanide oxide submicrospheres: PVP-assisted hydrothermal synthesis, size-control and luminescence properties." ChemPhysChem: a European journal of chemical physics and physical chemistry. 13 (10), pp. 2610-2614. https://doi.org/10.1002/cphc.201100806
One step molten salt synthesis of YVO4 nanoparticles and their photocatalytic properties under UV-Visible light
An, Xiaoxin, Wang, You, Deng, Jinxia, Chen, Jun, Yu, Ranbo and Xing, Xianran. 2014. "One step molten salt synthesis of YVO4 nanoparticles and their photocatalytic properties under UV-Visible light." Inorganic Chemistry Communications. 44, pp. 79-82. https://doi.org/10.1016/j.inoche.2014.03.010
A low-cost and large-scale synthesis of nano-zinc oxide from smithsonite
Zhang, Yucheng, Deng, Jinxia, Chen, Jun, Yu, Ranbo and Xing, Xianran. 2014. "A low-cost and large-scale synthesis of nano-zinc oxide from smithsonite." Inorganic Chemistry Communications. 43, pp. 138-141. https://doi.org/10.1016/j.inoche.2014.02.032
Quintuple-shelled Sno2 hollow microspheres with superior light scattering for high-performance dye-sensitized solar cells
Dong, Zhenghong, Ren, Hao, Hessel, Colin M., Wang, Jiangyan, Yu, Ranbo, Jin, Quan, Yang, Mei, Hu, Zhudong, Chen, Yunfa, Tang, Zhiyong, Zhao, Huijun and Wang, Dan. 2014. "Quintuple-shelled Sno2 hollow microspheres with superior light scattering for high-performance dye-sensitized solar cells." Advanced Materials. 26 (6), pp. 905-909. https://doi.org/10.1002/adma.201304010
Nd1-xCaxFeO3 (x = 0, 0.3) hollow core-shell microspheres for ethanol gas sensing
Wang, You, Wang, Yun, Chen, Jun, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2015. "Nd1-xCaxFeO3 (x = 0, 0.3) hollow core-shell microspheres for ethanol gas sensing." European Journal of Inorganic Chemistry. 2015 (35), pp. 5767-5772. https://doi.org/10.1002/ejic.201500869
Multi-shelled LiMn2O4 hollow microspheres as superior cathode materials for lithium-ion batteries
Wang, Feng, Wang, Jiangyan, Ren, Hao, Tang, Hongjie, Yu, Ranbo and Wang, Dan. 2016. "Multi-shelled LiMn2O4 hollow microspheres as superior cathode materials for lithium-ion batteries." Inorganic Chemistry Frontiers. 3 (3), pp. 365-369. https://doi.org/10.1039/c5qi00213c
ZnO-CdS@Cd heterostructure for effective photocatalytic hydrogen generation
Wang, Xuewen, Liu, Gang, Wang, Lianzhou, Chen, Zhi-Gang, Lu, Gao Qing and Cheng, Hui-Ming. 2012. "ZnO-CdS@Cd heterostructure for effective photocatalytic hydrogen generation." Advanced Energy Materials. 2 (1), pp. 42-46. https://doi.org/10.1002/aenm.201100528
Phase transformation and negative thermal expansion in TaVO5
Wang, Xiaowei, Huang, Qingzhen, Deng, Jinxia, Yu, Ranbo, Chen, Jun and Xing, Xianran. 2011. "Phase transformation and negative thermal expansion in TaVO5." Inorganic Chemistry: including bioinorganic chemistry. 50 (6), pp. 2685-2690. https://doi.org/10.1021/ic200003n
Facile solvothermal synthesis of gear-shaped submicrostructured Y2O3:Eu 3+ phosphor
Yan, Xuecheng, Yu, Ranbo, Wang, Dan, Deng, Jinxia, Chen, Jun and Xing, Xianran. 2011. "Facile solvothermal synthesis of gear-shaped submicrostructured Y2O3:Eu 3+ phosphor." Solid State Sciences. 13 (5), pp. 1060-1064. https://doi.org/10.1016/j.solidstatesciences.2011.01.019
The role of spontaneous polarization in the negative thermal expansion of tetragonal PbTiO3-based compounds
Chen, Jun, Nittala, Krishna, Forrester, Jennifer S., Jones, Jacob L., Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2011. "The role of spontaneous polarization in the negative thermal expansion of tetragonal PbTiO3-based compounds." Journal of the American Chemical Society. 133 (29), pp. 11114-11117. https://doi.org/10.1021/ja2046292
Facile molten salt synthesis of ordered perovskite Ba(Sr 1/3Nb 2/3)O3 powders
Deng, Jinxia, Li, Lihong, Chen, Jun, Yu, Ranbo and Xing, Xianran. 2012. "Facile molten salt synthesis of ordered perovskite Ba(Sr 1/3Nb 2/3)O3 powders." Inorganic Chemistry Communications. 21, pp. 92-95. https://doi.org/10.1016/j.inoche.2012.04.021
Morphology-tailored synthesis of flower-like Y 2O 3:Eu3+ microspheres
Yan, Xuecheng, Yu, Ranbo, Xu, Yali, Li, Li, Xu, Pengfei, Wang, Dan, Deng, Jinxia, Chen, Jun and Xing, Xianran. 2012. "Morphology-tailored synthesis of flower-like Y 2O 3:Eu3+ microspheres." Materials Research Bulletin. 47 (9), pp. 2135-2139. https://doi.org/10.1016/j.materresbull.2012.06.013
Rapid molten salt synthesis of isotropic negative thermal expansion ScF3
Hu, Lei, Chen, Jun, Fan, Longlong, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2014. "Rapid molten salt synthesis of isotropic negative thermal expansion ScF3." Journal of the American Ceramic Society. 97 (4), pp. 1009-1011. https://doi.org/10.1111/jace.12855
Large-scale synthesis of isotropic single-crystalline ScF3 cubes by hydrothermal method
Hu, Lei, Chen, Jun, Pan, Zhao, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2014. "Large-scale synthesis of isotropic single-crystalline ScF3 cubes by hydrothermal method." Journal of the American Ceramic Society. 97 (5), pp. 1386-1388. https://doi.org/10.1111/jace.12932
Zero thermal expansion and ferromagnetism in cubic sc1-xMxF3 (M = Ga, Fe) over a wide temperature range
Hu, Lei, Chen, Jun, Fan, Longlong, Ren, Yang, Rong, Yangchun, Pan, Zhao, Deng, Jinxia, Yu, Ranbo and Xing, Xianran. 2014. "Zero thermal expansion and ferromagnetism in cubic sc1-xMxF3 (M = Ga, Fe) over a wide temperature range." Journal of the American Chemical Society. 136 (39), pp. 13566-13569. https://doi.org/10.1021/ja5077487
Controlled synthesis and properties of porous Cu/CeO2 microspheres
Yao, Xiang, Yang, Xiaodan, Yu, Ranbo, Xu, Pengfei, Chen, Jun and Xing, Xianran. 2015. "Controlled synthesis and properties of porous Cu/CeO2 microspheres." Materials Research Bulletin. 61, pp. 22-25. https://doi.org/10.1016/j.materresbull.2014.09.083
Controllable assembly of CeO2 micro/nanospheres with adjustable size and their application in Cr(VI) adsorption
Sun, Jiajia, Wang, Chengrui, Zeng, Li, Xu, Pengfei, Yang, Xiaodan, Chen, Jun, Xing, Xianran, Jin, Quan and Yu, Ranbo. 2016. "Controllable assembly of CeO2 micro/nanospheres with adjustable size and their application in Cr(VI) adsorption." Materials Research Bulletin. 75, pp. 110-114. https://doi.org/10.1016/j.materresbull.2015.11.035
N,N-dimethylformamide-induced synthesis and photoluminescence of CePO4 and Ce0.95PO4:Tb0.05 with sphere-like nanostructures
Bao, Jinrong, Zhu, Xiaowei, Liu, Ying, Li, Wenxian and Yu, Ranbo. 2014. "N,N-dimethylformamide-induced synthesis and photoluminescence of CePO4 and Ce0.95PO4:Tb0.05 with sphere-like nanostructures." Materials Letters. 124, pp. 97-100. https://doi.org/10.1016/j.matlet.2014.03.014
Microstructure construction and composition modification of CeO2 macrospheres with superior performance
Jiang, Shuaiyu, Yang, Xiaodan, Chen, Jun, Xing, Xianran, Wang, Lianzhou and Yu, Ranbo. 2016. "Microstructure construction and composition modification of CeO2 macrospheres with superior performance." Inorganic Chemistry Frontiers. 3 (1), pp. 92-96. https://doi.org/10.1039/c5qi00140d
A novel and highly efficient photocatalyst based on P 25- graphdiyne nanocomposite
Wang, Shuo, Yi, Luoxin, Halpert, Jonathan E., Lai, Xiaoyong, Liu, Yuanyuan, Cao, Hongbin, Wang, Dan, Yu, Ranbo and Li, Yuliang. 2012. "A novel and highly efficient photocatalyst based on P 25- graphdiyne nanocomposite." Small. 8 (2), pp. 265-271. https://doi.org/10.1002/smll.201101686
Nanosized anatase TiO2 single crystals with tunable exposed (001) facets for enhanced energy conversion efficiency of dye-sensitized solar cells
Wu, Xia, Max Lu, Gao Qing, Wang, Lianzhou and Chen, Zhigang. 2011. "Nanosized anatase TiO2 single crystals with tunable exposed (001) facets for enhanced energy conversion efficiency of dye-sensitized solar cells." Advanced Functional Materials. 21 (21), pp. 4167-4172. https://doi.org/10.1002/adfm.201100828
Amino acid assisted synthesis of mesoporous TiO 2 nanocrystals for high performance dye-sensitized solar cells
Wu, Xia, Liu, Jian, Chen, Zhigang, Lu, Gaoqing, Wang, Lianzhou, Yang, Qihua and Li, Can. 2012. "Amino acid assisted synthesis of mesoporous TiO 2 nanocrystals for high performance dye-sensitized solar cells." Journal of Materials Chemistry. 22 (21), pp. 10438-10440. https://doi.org/10.1039/c2jm16762j
New electroless plating method for preparation of highly active Co-B catalysts for NaBH4 hydrolysis
Muir, Sean S., Chen, Zhigang, Wood, Barry J., Wang, Lianzhou, Lu, G. Q. (Max) and Yao, Xiangdong. 2014. "New electroless plating method for preparation of highly active Co-B catalysts for NaBH4 hydrolysis." International Journal of Hydrogen Energy. 39 (1), pp. 414-425. https://doi.org/10.1016/j.ijhydene.2013.10.022
Nitrogen doping in ion-exchangeable layered tantalate towards visible-light induced water oxidation
Zong, Xu, Sun, Chenghua, Chen, Zhigang, Mukherji, Aniruddh, Wu, Hao, Zou, Jin, Smith, Sean C., Lu, Gao Qing and Wang, Lianzhou. 2011. "Nitrogen doping in ion-exchangeable layered tantalate towards visible-light induced water oxidation." Chemical Communications. 47 (22), pp. 6293-6295. https://doi.org/10.1039/c0cc05440b
Photocatalytic water oxidation on F, N co-doped TiO2 with dominant exposed {001} facets under visible light
Zong, Xu, Xing, Zheng, Yu, Hua, Chen, Zhigang, Tang, Fengqiu, Zou, Jin, Lu, Gao Qing and Wang, Lianzhou. 2011. "Photocatalytic water oxidation on F, N co-doped TiO2 with dominant exposed {001} facets under visible light." Chemical Communications. 47 (42), pp. 11742-11744. https://doi.org/10.1039/c1cc14453g
A new type of carbon nitride-based polymer composite for enhanced photocatalytic hydrogen production
Xing, Zheng, Chen, Zhigang, Zong, Xu and Wang, Lianzhou. 2014. "A new type of carbon nitride-based polymer composite for enhanced photocatalytic hydrogen production." Chemical Communications. 50 (51), pp. 6762-6764. https://doi.org/10.1039/c4cc00397g
Study on the controllable scale-up growth of vertically-aligned carbon nanotube arrays
Ge, Lei, Chen, Jiuling, Chen, Jun, Zhu, Zhonghua and Rudolph, Victor. 2012. "Study on the controllable scale-up growth of vertically-aligned carbon nanotube arrays." Journal of Nanoscience and Nanotechnology. 12 (3), pp. 2722-2732. https://doi.org/10.1166/jnn.2012.5726
Reinforcement of natural rubber latex using lignocellulosic nanofibers isolated from spinifex grass
Hosseinmardi, Alireza, Annamalai, Pratheep K., Wang, Lianzhou, Martin, Darren and Amiralian, Nasim. 2017. "Reinforcement of natural rubber latex using lignocellulosic nanofibers isolated from spinifex grass." Nanoscale. 9 (27), pp. 9510-9519. https://doi.org/10.1039/c7nr02632c
Embeddable and locatable spinning
Xu, Weilin, Xia, Zhigang, Wang, Xin, Chen, Jun, Cui, Weigang, Ye, Wenxiang, Ding, Cailing and Wang, Xungai. 2011. "Embeddable and locatable spinning." Textile Research Journal. 81 (3), pp. 223-229. https://doi.org/10.1177/0040517510380780