Long-term geochemical evolution of acidic mine wastes under anaerobic conditions

Article

Lu, Wenzhou, Lin, Chuxia and Ma, Yingqun. 2013. "Long-term geochemical evolution of acidic mine wastes under anaerobic conditions ." Environmental Geochemistry and Health: official journal of the Society for Environmental Geochemistry and Health. 35 (4), pp. 523-533. https://doi.org/10.1007/s10653-013-9512-4
Article Title

Long-term geochemical evolution of acidic mine wastes under anaerobic conditions

ERA Journal ID36373
Article CategoryArticle
AuthorsLu, Wenzhou (Author), Lin, Chuxia (Author) and Ma, Yingqun (Author)
Journal TitleEnvironmental Geochemistry and Health: official journal of the Society for Environmental Geochemistry and Health
Journal Citation35 (4), pp. 523-533
Number of Pages11
Year2013
PublisherSpringer
Place of PublicationDordrecht, Netherlands
ISSN0269-4042
1573-2983
Digital Object Identifier (DOI)https://doi.org/10.1007/s10653-013-9512-4
Web Address (URL)http://link.springer.com/content/pdf/10.1007%2Fs10653-013-9512-4.pdf
Abstract

A nearly 5-year anaerobic incubation experiment was conducted to observe the geochemical evolution of an acidic mine waste. Long-term storage of the mine waste under strict anaerobic conditions caused marked increase in aqueous sulfur, while aqueous iron showed no remarkable change. Co-existing oxidation and reduction of elemental sulfur appeared to play a central role in controlling the evolutionary trends of aqueous sulfur and iron. Addition of organic matter increased the aqueous Fe concentration, possibly due to enhanced iron mobilization by microbial iron reduction and increased iron solubility by forming organically complexed Fe species. Further addition of CaCO3 resulted in immobilization of aqueous iron and sulfur due to elevated pH and gypsum formation. The chemical behaviors of environmentally significant metals were markedly affected by the added organic matter; Al, Cr, Cu, Ni and Zn tended to be immobilized probably due to elevated pH and complexation with insoluble organic molecules, while As and Pb tended to be mobilized. Jarosite exhibited high stability after nearly 5 years of anaerobic incubation and even under circumneutral pH conditions. Long-term weathering of aluminosilicate through acid attack raised pH, while continuous reaction between the added CaCO3 and mine waste-borne stored acid decreased pH.

Keywordsacidic mine waste; anaerobic condition; geochemical evolution; metal mobilization; sulfates; water parameters
ANZSRC Field of Research 2020410604. Soil chemistry and soil carbon sequestration (excl. carbon sequestration science)
400410. Wastewater treatment processes
370799. Hydrology not elsewhere classified
370104. Atmospheric composition, chemistry and processes
Public Notes

© 2013 Springer Science+Business Media Dordrecht. Published version deposited in accordance with the copyright policy of the publisher.

Byline AffiliationsMinistry of Environmental Protection, China
Australian Centre for Sustainable Catchments
Chinese Research Academy of Environmental Sciences, China
Institution of OriginUniversity of Southern Queensland
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