Fate and behavior of dissolved organic matter in a submerged anoxic-aerobic membrane bioreactor (MBR)
Article
Zhang, Dongqing, Trzcinski, Antoine Prandota, Luo, Jinxue, Stuckey, David C. and Tan, Soon Keat. 2018. "Fate and behavior of dissolved organic matter in a submerged anoxic-aerobic membrane bioreactor (MBR)." Environmental Science and Pollution Research. 25 (5), pp. 4289-4302. https://doi.org/10.1007/s11356-017-0586-x
| Article Title | Fate and behavior of dissolved organic matter in a submerged anoxic-aerobic membrane bioreactor (MBR) |
|---|---|
| ERA Journal ID | 5827 |
| Article Category | Article |
| Authors | Zhang, Dongqing (Author), Trzcinski, Antoine Prandota (Author), Luo, Jinxue (Author), Stuckey, David C. (Author) and Tan, Soon Keat (Author) |
| Journal Title | Environmental Science and Pollution Research |
| Journal Citation | 25 (5), pp. 4289-4302 |
| Number of Pages | 14 |
| Year | 2018 |
| Publisher | Springer |
| Place of Publication | Germany |
| ISSN | 0944-1344 |
| 1614-7499 | |
| Digital Object Identifier (DOI) | https://doi.org/10.1007/s11356-017-0586-x |
| Web Address (URL) | https://link.springer.com/article/10.1007%2Fs11356-017-0586-x |
| Abstract | In this study, the production, composition, and characteristics of dissolved organic matter (DOM) in an anoxic-aerobic submerged membrane bioreactor (MBR) were investigated. The average concentrations of proteins and carbohydrates in the MBR aerobic stage were 3.96 ± 0.28 and 8.36 ± 0.89 mg/L, respectively. After membrane filtration, these values decreased to 2.9 ± 0.2 and 2.8 ± 0.2 mg/L, respectively. High performance size exclusion chromatograph (HP-SEC) analysis indicated a bimodal molecular weight (MW) distribution of DOMs, and that the intensities of all the peaks were reduced in the MBR effluent compared to the influent. Three-dimensional fluorescence excitation emission matrix (FEEM) indicated that fulvic and humic acid-like substances were the predominant DOMs in biological treatment processes. Precise identification and characterization of low-MW DOMs was carried out using gas chromatography-mass spectrometry (GC-MS). The GC-MS analysis indicated that the highest peak numbers (170) were found in the anoxic stage, and 54 (32%) compounds were identified with a similarity greater than 80%. Alkanes (28), esters (11), and aromatics (7) were the main compounds detected. DOMs exhibited both biodegradable and recalcitrant characteristics. There were noticeable differences in the low-MW DOMs present down the treatment process train in terms of numbers, concentrations, molecular weight, biodegradability, and recalcitrance. |
| Keywords | dissolved organic matter (DOM); anoxic-aerobic MBR; fluorescence excitation emission matrix (EEM); gas chromatography-mass spectrometry (GC-MS) |
| ANZSRC Field of Research 2020 | 400409. Separation technologies |
| 401102. Environmentally sustainable engineering | |
| 410404. Environmental management | |
| Byline Affiliations | Nanyang Environment and Water Research Institute, Singapore |
| School of Civil Engineering and Surveying | |
| Chinese Academy of Sciences, China | |
| Imperial College London, United Kingdom | |
| Nanyang Technological University, Singapore | |
| Institution of Origin | University of Southern Queensland |
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