Unraveling electronic origins for boosting thermoelectric performance of p-type (Bi,Sb)2Te3

Article

Cheng, Rui, Ge, Haoran, Huang, Shengpu, Xie, Sen, Tong, Qiwei, Sang, Hao, Yan, Fan, Zhu, Liangyu, Wang, Rui, Liu, Yong, Hong, Min, Uher, Ctirad, Zhang, Qingjie, Liu, Wei and Tang, Xinfeng. 2024. "Unraveling electronic origins for boosting thermoelectric performance of p-type (Bi,Sb)2Te3." Science Advances. 10 (21). https://doi.org/10.1126/sciadv.adn9959
Article Title

Unraveling electronic origins for boosting thermoelectric performance of p-type (Bi,Sb)2Te3

ERA Journal ID211335
Article CategoryArticle
AuthorsCheng, Rui, Ge, Haoran, Huang, Shengpu, Xie, Sen, Tong, Qiwei, Sang, Hao, Yan, Fan, Zhu, Liangyu, Wang, Rui, Liu, Yong, Hong, Min, Uher, Ctirad, Zhang, Qingjie, Liu, Wei and Tang, Xinfeng
Journal TitleScience Advances
Journal Citation10 (21)
Article Numbereadn9959
Number of Pages9
Year2024
PublisherAmerican Association for the Advancement of Science (AAAS)
Place of PublicationUnited States
ISSN2375-2548
Digital Object Identifier (DOI)https://doi.org/10.1126/sciadv.adn9959
Web Address (URL)https://www.science.org/doi/10.1126/sciadv.adn9959
AbstractP-type Bi2-xSbxTe3 compounds are crucial for thermoelectric applications at room temperature, with Bi0.5Sb1.5Te3 demonstrating superior performance, attributed to its maximum density-of- states effective mass (m*). However, the underlying electronic origin remains obscure, impeding further performance optimization. Herein, we synthesized high-quality Bi2-xSbxTe3 (00 l) films and performed comprehensive angle-resolved photoemission spectroscopy (ARPES) measurements and band structure calculations to shed light on the electronic structures. ARPES results directly evidenced that the band convergence along the G-M direction contributes to the maximum m*of Bi0.5Sb1.5Te3. Moreover, strategic manipulation of intrinsic defects optimized the hole density of Bi0.5Sb1.5Te3, allowing the extra valence band along G-K to contribute to the electrical transport. The synergy of the above two aspects documented the electronic origins of the Bi0.5Sb1.5Te3's superior performance that resulted in an extraordinary power factor of ~5.5 milliwatts per meter per square kelvin. The study offers valuable guidance for further performance optimization of p-type Bi2-xSbxTe3.
Contains Sensitive ContentDoes not contain sensitive content
ANZSRC Field of Research 2020401605. Functional materials
Byline AffiliationsWuhan University of Technology, China
Chongqing University, China
Wuhan University, China
School of Engineering
Centre for Future Materials
University of Michigan, United States
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High-Performance PEDOT: PSS Flexible Thermoelectric Materials and Their Devices by Triple Post-Treatments
Xu, Shengduo, Hong, Min, Shi, Xiao-Lei, Wang, Yuan, Ge, Lei, Bai, Yang, Wang, Lianzhou, Dargusch, Matthew, Zou, Jin and Chen, Zhi-Gang. 2019. "High-Performance PEDOT: PSS Flexible Thermoelectric Materials and Their Devices by Triple Post-Treatments." Chemisty of Materials. 31 (14), pp. 5238-5244. https://doi.org/10.1021/acs.chemmater.9b01500
Exploring the underlying mechanisms behind the increased far infrared radiation properties of perovskite-type Ce/Mn co-doped ceramics
Deng, Yi, Zhang, Kewei, Shi, Xiuyuan, Dong, Taosheng, Yang, Lei, Yang, Weizhong, Hong, Min, Wang, Yuan, Dargusch, Matthew and Chen, Zhi-Gang. 2019. "Exploring the underlying mechanisms behind the increased far infrared radiation properties of perovskite-type Ce/Mn co-doped ceramics." Materials Research Bulletin. 109, pp. 233-239. https://doi.org/10.1016/j.materresbull.2018.09.042
Strong phonon–phonon interactions securing extraordinary thermoelectric Ge1–xSbxTe with Zn-alloying-induced band alignment
Hong, Min, Wang, Yuan, Feng, Tianli, Sun, Qiang, Xu, Shengduo, Matsumura, Syo, Pantelides, Sokrates T., Zou, Jin and Chen, Zhi-Gang. 2019. "Strong phonon–phonon interactions securing extraordinary thermoelectric Ge1–xSbxTe with Zn-alloying-induced band alignment." Journal of the American Chemical Society. 141 (4), pp. 1742-1748. https://doi.org/10.1021/jacs.8b12624
High Thermoelectric Performance in p-type Polycrystalline Cd-doped SnSe Achieved by a Combination of Cation Vacancies and Localized Lattice Engineering
Shi, Xiaolei, Wu, Angyin, Feng, Tianli, Zheng, Kun, Liu, Weidi, Sun, Qiang, Hong, Min, Pantelides, Sokrates T., Chen, Zhi-Gang and Zou, Jin. 2019. "High Thermoelectric Performance in p-type Polycrystalline Cd-doped SnSe Achieved by a Combination of Cation Vacancies and Localized Lattice Engineering." Advanced Energy Materials. 9 (11), pp. 1-15. https://doi.org/10.1002/aenm.201803242
High Porosity in Nanostructured n-Type Bi2Te3 Obtaining Ultralow Lattice Thermal Conductivity
Wang, Yuan, Liu, Wei-Di, Gao, Han, Wang, Li-Jun, Li, Meng, Shi, Xiao-Lei, Hong, Min, Wang, Hao, Zou, Jin and Chen, Zhi-Gang. 2019. "High Porosity in Nanostructured n-Type Bi2Te3 Obtaining Ultralow Lattice Thermal Conductivity ." ACS Applied Materials and Interfaces. 11 (34), pp. 31237-31244. https://doi.org/10.1021/acsami.9b12079
Real-time observation of the thermally-induced phase transformation in GeTe and its thermal expansion properties
Tran, Xuan Quy, Hong, Min, Maeno, Hiroshi, Kawami, Youichirou, Toriyama, Takaaki, Jack, Kevin, Chen, Zhi-Gang, Zou, Jin, Matsumura, Syo and Dargusch, Matthew S.. 2019. "Real-time observation of the thermally-induced phase transformation in GeTe and its thermal expansion properties." Acta Materialia. 165, pp. 327-335. https://doi.org/10.1016/j.actamat.2018.11.059
Thermoelectric GeTe with Diverse Degrees of Freedom Having Secured Superhigh Performance
Hong, Min, Zou, Jin and Chen, Zhi-Gang. 2019. "Thermoelectric GeTe with Diverse Degrees of Freedom Having Secured Superhigh Performance." Advanced Materials. 31 (14), pp. 1-23. https://doi.org/10.1002/adma.201807071
High thermoelectric performance in sintered octahedron-shaped Sn(CdIn)xTe1+2x microcrystals
Moshwan, Raza, Shi, Xiao-Lei, Liu, Wei-Di, Yang, Lei, Wang, Yuan, Hong, Min, Auchterlonie, Graeme, Zou, Jin and Chen, Zhi-Gang. 2018. "High thermoelectric performance in sintered octahedron-shaped Sn(CdIn)xTe1+2x microcrystals." ACS Applied Materials and Interfaces. 10 (45), pp. 38944-38952. https://doi.org/10.1021/acsami.8b14233
Dual Ag/ZnO-decorated micro-/nanoporous sulfonated polyetheretherketone with superior antibacterial capability and biocompatibility via layer-by-layer self-assembly strategy
Deng, Yi, Yang, Lei, Huang, Xiaobing, Chen, Junhong, Shi, Xiuyuan, Yang, Weizhong, Hong, Min, Wang, Yuan, Dargusch, Matthew and Chen, Zhi-Gang. 2018. "Dual Ag/ZnO-decorated micro-/nanoporous sulfonated polyetheretherketone with superior antibacterial capability and biocompatibility via layer-by-layer self-assembly strategy." Macromolecular Bioscience. 18 (7), pp. 1-12. https://doi.org/10.1002/mabi.201800028
Achieving high thermoelectric performance of Ni/Cu modified Bi0.5Sb1.5Te3 composites by a facile electroless plating
Huang, Zhong-Yue, Zhang, He, Yang, Lei, Zhu, Bin, Zheng, Kun, Hong, Min, Yu, Yuan, Zu, Fang-Qiu, Zou, Jin and Chen, Zhi-Gang. 2018. "Achieving high thermoelectric performance of Ni/Cu modified Bi0.5Sb1.5Te3 composites by a facile electroless plating." Materials Today Energy. 9, pp. 383-390. https://doi.org/10.1016/j.mtener.2018.06.011
Ag doping induced abnormal lattice thermal conductivity in Cu2Se
Liu, Weidi, Shi, Xiaolei, Hong, Min, Yang, Lei, Moshwan, Raza, Chen, Zhi-Gang and Zou, Jin. 2018. "Ag doping induced abnormal lattice thermal conductivity in Cu2Se." Journal of Materials Chemistry C. 6 (48), pp. 13225-13231. https://doi.org/10.1039/c8tc04129f
Enhancing thermoelectric performance of (Cu1-xAgx)2Se via CuAgSe secondary phase and porous design
Liu, Weidi, Shi, Xiaolei, Moshwan, Raza, Hong, Min, Yang, Lei, Chen, Zhi-Gang and Zou, Jin. 2018. "Enhancing thermoelectric performance of (Cu1-xAgx)2Se via CuAgSe secondary phase and porous design." Sustainable Materials and Technologies. 17, pp. 1-8. https://doi.org/10.1016/j.susmat.2018.e00076
Atomic Insights into Phase Evolution in Ternary Transition-Metal Dichalcogenides Nanostructures
Zou, Yi-Chao, Chen, Zhi-Gang, Aso, Kohei, Zhang, Chenxi, Kong, Fantai, Hong, Min, Matsumura, Syo, Cho, Kyeongjae and Zou, Jin. 2018. "Atomic Insights into Phase Evolution in Ternary Transition-Metal Dichalcogenides Nanostructures." Small. 14 (22), pp. 1-6. https://doi.org/10.1002/smll.201800780
Boosting the thermoelectric performance of p-type heavily Cu-doped polycrystalline SnSe via inducing intensive crystal imperfections and defect phonon scattering
Shi, Xiaolei, Zheng, Kun, Hong, Min, Liu, Weidi, Moshwan, Raza, Wang, Yuan, Qu, Xianlin, Chen, Zhi-Gang and Zou, Jin. 2018. "Boosting the thermoelectric performance of p-type heavily Cu-doped polycrystalline SnSe via inducing intensive crystal imperfections and defect phonon scattering." Chemical Science. 9 (37), pp. 7376-7389. https://doi.org/10.1039/C8SC02397b
Sustainable utilization of municipal solid waste i incineration fly ash for ceramic bricks with eco-friendly biosafety
Deng, Yi, Gong, B., Chao, Y., Dong, T., Yang, W., Hong, Min, Shi, X., Wang, G., Jin, Y. and Chen, Z.-G.. 2018. "Sustainable utilization of municipal solid waste i incineration fly ash for ceramic bricks with eco-friendly biosafety." Materials Today Sustainability. 1-2, pp. 32-38. https://doi.org/10.1016/j.mtsust.2018.11.002
Self-assembled 3D flower-like hierarchical Ti-doped Cu3SbSe4 microspheres with ultralow thermal conductivity and high zT
Zhou, Tian, Wang, Lijun, Zheng, Shuqi, Hong, Min, Fang, Teng, Bai, Peng-Peng, Chang, Siyi, Cui, Wenlin, Shi, Xiaolei, Zhao, Huaizhou and Chen, Zhi-Gang. 2018. "Self-assembled 3D flower-like hierarchical Ti-doped Cu3SbSe4 microspheres with ultralow thermal conductivity and high zT." Nano Energy. 49, pp. 221-229. https://doi.org/10.1016/j.nanoen.2018.04.035
Nano-scale dislocations induced by self-vacancy engineering yielding extraordinary n-type thermoelectric Pb0.96-yInySe
Hong, Min, Chen, Zhi-Gang, Matsumura, Syo and Zou, Jin. 2018. "Nano-scale dislocations induced by self-vacancy engineering yielding extraordinary n-type thermoelectric Pb0.96-yInySe." Nano Energy. 50, pp. 785-793. https://doi.org/10.1016/j.nanoen.2018.06.030
Arrays of planar vacancies in superior thermoelectric Ge1−x−yCdxBiyTe with band convergence
Hong, Min, Wang, Yuan, Liu, Weidi, Matsumura, Syo, Wang, Hao, Zou, Jin and Chen, Zhi-Gang. 2018. "Arrays of planar vacancies in superior thermoelectric Ge1−x−yCdxBiyTe with band convergence." Advanced Energy Materials. 8 (30), pp. 1-10. https://doi.org/10.1002/aenm.201801837
Realizing zT of 2.3 in Ge1−x−ySbxInyTe via Reducing the Phase-Transition Temperature and Introducing Resonant Energy Doping
Hong, Min, Chen, Zhi-Gang, Yang, Lei, Zou, Yi-Chao, Dargusch, Matthew, Wang, Hao and Zou, Jin. 2018. "Realizing zT of 2.3 in Ge1−x−ySbxInyTe via Reducing the Phase-Transition Temperature and Introducing Resonant Energy Doping." Advanced Materials. 30 (11), pp. 1-8. https://doi.org/10.1002/adma.201705942
Achieving zT > 2 in p-Type AgSbTe2−xSex alloys via exploring the extra light valence band and introducing dense stacking faults
Hong, Min, Chen, Zhi-Gang, Yang, Lei, Liao, Zhi-Ming, Zou, Yi-Chao, Chen, Yan-Hui, Matsumura, Syo and Zou, Jin. 2018. "Achieving zT > 2 in p-Type AgSbTe2−xSex alloys via exploring the extra light valence band and introducing dense stacking faults." Advanced Energy Materials. 8 (9), pp. 1-7. https://doi.org/10.1002/aenm.201702333
BixSb2_xTe3 nanoplates with enhanced thermoelectric performance due to sufficiently decoupled electronic transport properties and strong wide-frequency phonon scatterings
Hong, Min, Chen, Zhi G., Yang, Lei and Zou, Jin. 2016. "BixSb2_xTe3 nanoplates with enhanced thermoelectric performance due to sufficiently decoupled electronic transport properties and strong wide-frequency phonon scatterings." Nano Energy. 20, pp. 144-155. https://doi.org/10.1016/j.nanoen.2015.12.009
Enhancing the thermoelectric performance of SnSe1-xTex nanoplates through band engineering
Hong, Min, Chen, Zhi-Gang, Yang, Lei, Chasapis, Thomas C., Kang, Stephen Dongmin, Zou, Yichao, Auchterlonie, Graeme John, Kanatzidis, Mercouri G., Snyder, G. Jeffrey and Zou, Jin. 2017. "Enhancing the thermoelectric performance of SnSe1-xTex nanoplates through band engineering." Journal of Materials Chemistry A. 5 (21), pp. 10713-10721. https://doi.org/10.1039/c7ta02677c
Fundamental and progress of Bi2Te3-based thermoelectric materials
Hong, Min, Chen, Zhigang and Zou, Jin. 2018. "Fundamental and progress of Bi2Te3-based thermoelectric materials." Chinese Physics B. 27 (4), pp. 1-25. https://doi.org/10.1088/1674-1056/27/4/048403
Achieving high Figure of Merit in p-type polycrystalline Sn0.98Se via self-doping and anisotropy-strengthening
Shi, Xiaolei, Chen, Zhi-Gang, Liu, Weidi, Yang, Lei, Hong, Min, Moshwan, Raza, Huang, Liqing and Zou, Jin. 2018. "Achieving high Figure of Merit in p-type polycrystalline Sn0.98Se via self-doping and anisotropy-strengthening." Energy Storage Materials. 10, pp. 130-138. https://doi.org/10.1016/j.ensm.2017.08.014
Scalable growth of high mobility dirac semimetal Cd3As2 microbelts
Chen, Zhi Gang, Zhang, Cheng, Zou, Yichao, Zhang, Enze, Yang, Lei, Hong, Min, Xiu, Faxian and Zou, Jin. 2015. "Scalable growth of high mobility dirac semimetal Cd3As2 microbelts." Nano Letters: a journal dedicated to nanoscience and nanotechnology. 15 (9), pp. 5830-5834. https://doi.org/10.1021/acs.nanolett.5b01885
Limit of zT enhancement in rocksalt structured chalcogenides by band convergence
Hong, Min, Chen, Zhi-Gang, Pei, Yanzhong, Yang, Lei and Zou, Jin. 2016. "Limit of zT enhancement in rocksalt structured chalcogenides by band convergence." Physical Review B: Covering condensed matter and materials physics. 94 (16). https://doi.org/10.1103/PhysRevB.94.161201
Enhancing thermoelectric performance of Bi2Te3-based nanostructures through rational structure design
Hong, Min, Chen, Zhi-Gang, Yang, Lei and Zou, Jin. 2016. "Enhancing thermoelectric performance of Bi2Te3-based nanostructures through rational structure design." Nanoscale. 8 (16), pp. 8681-8686. https://doi.org/10.1039/c6nr00719h
Co-doped Sb2Te3 paramagnetic nanoplates
Yang, Lei, Chen, Zhi-Gang, Nie, Tianxiao, Han, Guang, Zhang, Zhi, Hong, Min, Wang, Kang L. and Zou, Jin. 2016. "Co-doped Sb2Te3 paramagnetic nanoplates." Journal of Materials Chemistry C. 4 (3), pp. 521-525. https://doi.org/10.1039/c5tc03767k
Te-Doped Cu2Se nanoplates with a high average thermoelectric figure of merit
Yang, Lei, Chen, Zhi-Gang, Han, Guang, Hong, Min, Huang, Liqing and Zou, Jin. 2016. "Te-Doped Cu2Se nanoplates with a high average thermoelectric figure of merit." Journal of Materials Chemistry A. 4 (23), pp. 9213-9219. https://doi.org/10.1039/c6ta02998a
Rational design of Bi2Te3 polycrystalline whiskers for thermoelectric applications
Han, Guang, Chen, Zhi Gang, Yang, Lei, Hong, Min, Drennan, John and Zou, Jin. 2015. "Rational design of Bi2Te3 polycrystalline whiskers for thermoelectric applications." ACS Applied Materials and Interfaces. 7 (1), pp. 989-995. https://doi.org/10.1021/am5078528
Enhanced Thermoelectric Performance of Nanostructured Bi2Te3 through Significant Phonon Scattering
Yang, Lei, Chen, Zhi Gang, Hong, Min, Han, Guang and Zou, Jin. 2015. "Enhanced Thermoelectric Performance of Nanostructured Bi2Te3 through Significant Phonon Scattering." ACS Applied Materials and Interfaces. 7 (42), pp. 23694-23699. https://doi.org/10.1021/acsami.5b07596
n-type Bi2Te3-xSex nanoplates with enhanced thermoelectric efficiency driven by wide-frequency phonon scatterings and synergistic carrier scatterings
Hong, Min, Chasapis, Thomas C., Chen, Zhi Gang, Yang, Lei, Kanatzidis, Mercouri G., Snyder, G. Jeffrey and Zou, Jin. 2016. "n-type Bi2Te3-xSex nanoplates with enhanced thermoelectric efficiency driven by wide-frequency phonon scatterings and synergistic carrier scatterings." ACS Nano. 10 (4), pp. 4719-4727. https://doi.org/10.1021/acsnano.6b01156
Enhanced thermoelectric performance of ultrathin Bi2Se3 nanosheets through thickness control
Hong, Min, Chen, Zhi-Gang, Yang, Lei, Han, Guang and Zou, Jin. 2015. "Enhanced thermoelectric performance of ultrathin Bi2Se3 nanosheets through thickness control." Advanced Electronic Materials. 1 (6). https://doi.org/10.1002/aelm.201500025
High-performance thermoelectric Cu2Se nanoplates through nanostructure engineering
Yang, Lei, Chen, Zhi-Gang, Han, Guang, Hong, Min, Zou, Yichao and Zou, Jin. 2015. "High-performance thermoelectric Cu2Se nanoplates through nanostructure engineering." Nano Energy. 16, pp. 367-374. https://doi.org/10.1016/j.nanoen.2015.07.012
Impacts of Cu deficiency on the thermoelectric properties of Cu2-XSe nanoplates
Yang, Lei, Chen, Zhi-Gang, Han, Guang, Hong, Min and Zou, Jin. 2016. "Impacts of Cu deficiency on the thermoelectric properties of Cu2-XSe nanoplates." Acta Materialia. 113, pp. 140-146. https://doi.org/10.1016/j.actamat.2016.04.050
n-type Bi-doped PbTe nanocubes with enhanced thermoelectric performance
Yang, Lei, Chen, Zhi-Gang, Hong, Min, Wang, Lihua, Kong, Deli, Huang, Liqing, Han, Guang, Zou, Yichao, Dargusch, Matthew and Zou, Jin. 2017. "n-type Bi-doped PbTe nanocubes with enhanced thermoelectric performance." Nano Energy. 31, pp. 105-112. https://doi.org/10.1016/j.nanoen.2016.11.027